Impact of Fluoroalkylation on the n-Type Charge Transport of Two Naphthodithiophene Diimide Derivatives.

DFT charge mobility anisotropy charge transfer charge transport dynamic disorder electron-phonon coupling n-type organic crystals organic semiconductors quantum chemistry

Journal

Molecules (Basel, Switzerland)
ISSN: 1420-3049
Titre abrégé: Molecules
Pays: Switzerland
ID NLM: 100964009

Informations de publication

Date de publication:
06 Jul 2021
Historique:
received: 11 06 2021
revised: 03 07 2021
accepted: 04 07 2021
entrez: 24 7 2021
pubmed: 25 7 2021
medline: 25 7 2021
Statut: epublish

Résumé

In this work, we investigate two recently synthesized naphthodithiophene diimide (NDTI) derivatives featuring promising n-type charge transport properties. We analyze the charge transport pathways and model charge mobility with the non-adiabatic hopping mechanism using the Marcus-Levich-Jortner rate constant formulation, highlighting the role of fluoroalkylated substitution in α (

Identifiants

pubmed: 34299394
pii: molecules26144119
doi: 10.3390/molecules26144119
pmc: PMC8307299
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Subventions

Organisme : Deutsche Forschungsgemeinschaft
ID : FA 1502/1-1

Références

Chem Commun (Camb). 2016 Dec 20;53(1):188-191
pubmed: 27917425
Acc Chem Res. 2009 Oct 20;42(10):1669-78
pubmed: 19645446
J Chem Theory Comput. 2018 Oct 9;14(10):5273-5289
pubmed: 30176213
Chem Rev. 2007 Apr;107(4):926-52
pubmed: 17378615
Chem Soc Rev. 2014 Apr 21;43(8):2662-79
pubmed: 24394992
J Am Chem Soc. 2009 Apr 22;131(15):5586-608
pubmed: 19331320
Chem Rev. 2004 Nov;104(11):4971-5004
pubmed: 15535639
Angew Chem Int Ed Engl. 2014 Jul 14;53(29):7428-48
pubmed: 24961807
Acc Chem Res. 2011 Jul 19;44(7):501-10
pubmed: 21615105
Phys Chem Chem Phys. 2014 Oct 21;16(39):21550-8
pubmed: 25188414
J Am Chem Soc. 2010 Mar 24;132(11):3697-9
pubmed: 20187650
Adv Mater. 2012 Jul 17;24(27):3678-84
pubmed: 22689261
Chem Rec. 2015 Feb;15(1):175-88
pubmed: 25346498
J Phys Chem B. 2010 Apr 29;114(16):5327-34
pubmed: 20373750
J Am Chem Soc. 2008 Sep 17;130(37):12377-84
pubmed: 18715006
Adv Mater. 2018 Jul 18;:e1801079
pubmed: 30022536
Phys Chem Chem Phys. 2010 Apr 7;12(13):3309-14
pubmed: 20237724
Phys Chem Chem Phys. 2019 Jan 23;21(4):2057-2068
pubmed: 30638227
Phys Chem Chem Phys. 2015 Jun 14;17(22):14342-54
pubmed: 25573447
J Chem Phys. 2016 Feb 7;144(5):054103
pubmed: 26851904
J Chem Phys. 2011 Aug 28;135(8):084701
pubmed: 21895208
Chem Soc Rev. 2011 May;40(5):2347-58
pubmed: 21409232
ACS Appl Mater Interfaces. 2014 Oct 22;6(20):18098-103
pubmed: 25248967
Sci Adv. 2020 May 01;6(18):eaaz0632
pubmed: 32494668
Nat Commun. 2019 Aug 26;10(1):3843
pubmed: 31451687
J Am Chem Soc. 2012 Mar 7;134(9):4084-7
pubmed: 22352880
J Am Chem Soc. 2009 May 13;131(18):6591-8
pubmed: 19374415
Phys Chem Chem Phys. 2017 May 31;19(21):13978-13993
pubmed: 28516987
Phys Rev Lett. 2006 Mar 3;96(8):086601
pubmed: 16606209
J Am Chem Soc. 2011 Nov 16;133(45):18054-7
pubmed: 21999401
J Phys Chem A. 2006 Mar 23;110(11):4065-70
pubmed: 16539430
J Chem Theory Comput. 2018 Jul 10;14(7):3752-3762
pubmed: 29851487
J Phys Chem A. 2006 May 18;110(19):6356-64
pubmed: 16686472
Adv Mater. 2020 Mar;32(10):e1905909
pubmed: 31965662
Adv Mater. 2019 Oct;31(43):e1902407
pubmed: 31512304
Adv Mater. 2019 Nov;31(45):e1804699
pubmed: 30300439
ACS Appl Mater Interfaces. 2020 May 20;12(20):23225-23235
pubmed: 32252522
Proc Natl Acad Sci U S A. 2005 Mar 8;102(10):3552-7
pubmed: 15738409
J Chem Phys. 2014 Mar 14;140(10):104105
pubmed: 24628150
Adv Mater. 2014 Feb 26;26(8):1254-60
pubmed: 24338981
Chem Rev. 2017 Aug 9;117(15):10319-10357
pubmed: 28644623
J Am Chem Soc. 2013 Aug 7;135(31):11445-8
pubmed: 23879366
J Chem Phys. 2008 Jan 21;128(3):034701
pubmed: 18205512
J Am Chem Soc. 2009 Jan 14;131(1):8-9
pubmed: 19090656
Chemphyschem. 2009 Sep 14;10(13):2265-73
pubmed: 19637205
J Am Chem Soc. 2010 Oct 20;132(41):14437-46
pubmed: 20866074
J Am Chem Soc. 2013 Feb 13;135(6):2338-49
pubmed: 23327415
Phys Chem Chem Phys. 2008 Oct 21;10(39):5941-52
pubmed: 18825280
Org Biomol Chem. 2012 Aug 28;10(32):6455-68
pubmed: 22782711
Adv Mater. 2016 Dec;28(48):10764-10771
pubmed: 27787927
Phys Chem Chem Phys. 2010 Sep 28;12(36):11103-13
pubmed: 20689881
ACS Appl Mater Interfaces. 2018 Sep 26;10(38):32444-32453
pubmed: 30168319
Nature. 2000 Mar 30;404(6777):478-81
pubmed: 10761911
Acc Chem Res. 2021 Feb 2;54(3):642-653
pubmed: 33289387
J Am Chem Soc. 2006 Aug 2;128(30):9882-6
pubmed: 16866546
Nat Commun. 2016 Mar 10;7:10908
pubmed: 26961271

Auteurs

Gaetano Ricci (G)

Dipartimento di Chimica "Giacomo Ciamician", Università di Bologna, Via F. Selmi, 2, 40126 Bologna, Italy.

Sofia Canola (S)

Dipartimento di Chimica "Giacomo Ciamician", Università di Bologna, Via F. Selmi, 2, 40126 Bologna, Italy.

Yasi Dai (Y)

Dipartimento di Chimica "Giacomo Ciamician", Università di Bologna, Via F. Selmi, 2, 40126 Bologna, Italy.

Daniele Fazzi (D)

Institut für Physikalische Chemie, Department für Chemie, Universität zu Köln, Greinstr. 4-6, D-50939 Köln, Germany.

Fabrizia Negri (F)

Dipartimento di Chimica "Giacomo Ciamician", Università di Bologna, Via F. Selmi, 2, 40126 Bologna, Italy.
INSTM, UdR Bologna, Via F. Selmi, 2, 40126 Bologna, Italy.

Classifications MeSH