Moving Dirac nodes by chemical substitution.

Dirac semi-metals correlated electronic systems functional topological materials

Journal

Proceedings of the National Academy of Sciences of the United States of America
ISSN: 1091-6490
Titre abrégé: Proc Natl Acad Sci U S A
Pays: United States
ID NLM: 7505876

Informations de publication

Date de publication:
17 Aug 2021
Historique:
entrez: 13 8 2021
pubmed: 14 8 2021
medline: 14 8 2021
Statut: ppublish

Résumé

Dirac fermions play a central role in the study of topological phases, for they can generate a variety of exotic states, such as Weyl semimetals and topological insulators. The control and manipulation of Dirac fermions constitute a fundamental step toward the realization of novel concepts of electronic devices and quantum computation. By means of Angle-Resolved Photo-Emission Spectroscopy (ARPES) experiments and ab initio simulations, here, we show that Dirac states can be effectively tuned by doping a transition metal sulfide, [Formula: see text], through Co/Ni substitution. The symmetry and chemical characteristics of this material, combined with the modification of the charge-transfer gap of [Formula: see text] across its phase diagram, lead to the formation of Dirac lines, whose position in k-space can be displaced along the [Formula: see text] symmetry direction and their form reshaped. Not only does the doping x tailor the location and shape of the Dirac bands, but it also controls the metal-insulator transition in the same compound, making [Formula: see text] a model system to functionalize Dirac materials by varying the strength of electron correlations.

Identifiants

pubmed: 34385327
pii: 2108617118
doi: 10.1073/pnas.2108617118
pmc: PMC8379913
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Déclaration de conflit d'intérêts

The authors declare no competing interest.

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Auteurs

Niloufar Nilforoushan (N)

Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS, 91405 Orsay, France; niloufar.nilforoushan@phys.ens.fr michele.casula@upmc.fr marino.marsi@universite-paris-saclay.fr.

Michele Casula (M)

Institut de Minéralogie de Physique des Matériaux et de Cosmochimie, Sorbonne Université, CNRS UMR 7590, Museum National d'Histoire Naturelle, 75252 Paris, France; niloufar.nilforoushan@phys.ens.fr michele.casula@upmc.fr marino.marsi@universite-paris-saclay.fr.

Adriano Amaricci (A)

Istituto Officina dei Materiali, Consiglio Nazionale delle Ricerche, 34149 Trieste, Italy.
International School for Advanced Studies (SISSA), 34136 Trieste, Italy.

Marco Caputo (M)

Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS, 91405 Orsay, France.
Elettra Sincrotrone Trieste, Area Science Park, 34149 Trieste, Italy.

Jonathan Caillaux (J)

Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS, 91405 Orsay, France.

Lama Khalil (L)

Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS, 91405 Orsay, France.
Synchrotron SOLEIL, Gif-sur-Yvette F-91192, France.

Evangelos Papalazarou (E)

Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS, 91405 Orsay, France.

Pascal Simon (P)

Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS, 91405 Orsay, France.

Luca Perfetti (L)

Laboratoire des Solides Irradiés, CEA/DRF/lRAMIS, CNRS, Ecole Polytechnique, Institut Polytechnique de Paris, 91128 Palaiseau, France.

Ivana Vobornik (I)

Istituto Officina dei Materiali, Consiglio Nazionale delle Ricerche, 34149 Trieste, Italy.

Pranab Kumar Das (PK)

Istituto Officina dei Materiali, Consiglio Nazionale delle Ricerche, 34149 Trieste, Italy.
International Centre for Theoretical Physics, 34151 Trieste, Italy.

Jun Fujii (J)

Istituto Officina dei Materiali, Consiglio Nazionale delle Ricerche, 34149 Trieste, Italy.

Alexei Barinov (A)

Elettra Sincrotrone Trieste, Area Science Park, 34149 Trieste, Italy.

David Santos-Cottin (D)

Institut de Minéralogie de Physique des Matériaux et de Cosmochimie, Sorbonne Université, CNRS UMR 7590, Museum National d'Histoire Naturelle, 75252 Paris, France.

Yannick Klein (Y)

Institut de Minéralogie de Physique des Matériaux et de Cosmochimie, Sorbonne Université, CNRS UMR 7590, Museum National d'Histoire Naturelle, 75252 Paris, France.

Michele Fabrizio (M)

International School for Advanced Studies (SISSA), 34136 Trieste, Italy.

Andrea Gauzzi (A)

Institut de Minéralogie de Physique des Matériaux et de Cosmochimie, Sorbonne Université, CNRS UMR 7590, Museum National d'Histoire Naturelle, 75252 Paris, France.

Marino Marsi (M)

Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS, 91405 Orsay, France; niloufar.nilforoushan@phys.ens.fr michele.casula@upmc.fr marino.marsi@universite-paris-saclay.fr.

Classifications MeSH