Identifying Reactive Sites and Surface Traps in Chalcopyrite Photocathodes.
chalcopyrite
density functional theory
photoelectrochemistry
spectroelectrochemistry
water splitting
Journal
Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543
Informations de publication
Date de publication:
25 Oct 2021
25 Oct 2021
Historique:
revised:
06
08
2021
received:
06
07
2021
pubmed:
25
8
2021
medline:
25
8
2021
entrez:
24
8
2021
Statut:
ppublish
Résumé
Gathering information on the atomic nature of reactive sites and trap states is key to fine tuning catalysis and suppressing deleterious surface voltage losses in photoelectrochemical technologies. Here, spectroelectrochemical and computational methods were combined to investigate a model photocathode from the promising chalcopyrite family: CuIn
Identifiants
pubmed: 34428331
doi: 10.1002/anie.202108994
pmc: PMC8597141
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
23651-23655Subventions
Organisme : schweizerischer nationalfonds zur förderung der wissenschaftlichen forschung
ID : PZENP2_166871
Organisme : schweizerischer nationalfonds zur förderung der wissenschaftlichen forschung
ID : PP00P2_157615
Organisme : gaznat-epfl research program
Organisme : china scholarship council
ID : CSC201806160172
Organisme : strategic japanese-swiss science and technology program
ID : 514259
Informations de copyright
© 2021 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH.
Références
J Am Chem Soc. 2005 Apr 20;127(15):5308-9
pubmed: 15826154
J Am Chem Soc. 2012 Mar 7;134(9):4294-302
pubmed: 22303953
J Am Chem Soc. 2016 Dec 7;138(48):15673-15681
pubmed: 27934030
Angew Chem Int Ed Engl. 2021 Feb 19;60(8):4034-4037
pubmed: 33185337
J Am Chem Soc. 2013 Mar 13;135(10):3733-5
pubmed: 23437875
Chem Sci. 2017 May 1;8(5):3712-3719
pubmed: 28580106
Nat Commun. 2020 Jul 20;11(1):3634
pubmed: 32686684
Langmuir. 2014 Jul 1;30(25):7593-600
pubmed: 24940629
J Am Chem Soc. 2012 Oct 10;134(40):16693-700
pubmed: 22950478
Angew Chem Int Ed Engl. 2021 Feb 15;60(7):3504-3509
pubmed: 33105064
Nat Commun. 2017 Feb 24;8:14280
pubmed: 28233785
J Am Chem Soc. 2020 Apr 29;142(17):7795-7802
pubmed: 32270679
Angew Chem Int Ed Engl. 2020 Oct 19;59(43):18990-18995
pubmed: 32666681
Sci Rep. 2018 Mar 26;8(1):5182
pubmed: 29581436
Angew Chem Int Ed Engl. 2021 Oct 25;60(44):23651-23655
pubmed: 34428331
ACS Appl Mater Interfaces. 2018 Jun 13;10(23):19573-19579
pubmed: 29767955