MIXed plastics biodegradation and UPcycling using microbial communities: EU Horizon 2020 project MIX-UP started January 2020.

Biobased plastic Depolymerisation Metabolic engineering Microbial consortia Mixed plastics valorisation PHA Plastic crisis Plastic recycling Polyhydroxyalkanoate Synthetic biology

Journal

Environmental sciences Europe
ISSN: 2190-4707
Titre abrégé: Environ Sci Eur
Pays: Germany
ID NLM: 101571842

Informations de publication

Date de publication:
2021
Historique:
received: 09 05 2021
accepted: 31 07 2021
entrez: 30 8 2021
pubmed: 31 8 2021
medline: 31 8 2021
Statut: ppublish

Résumé

This article introduces the EU Horizon 2020 research project MIX-UP, "Mixed plastics biodegradation and upcycling using microbial communities". The project focuses on changing the traditional linear value chain of plastics to a sustainable, biodegradable based one. Plastic mixtures contain five of the top six fossil-based recalcitrant plastics [polyethylene (PE), polyurethane (PUR), polypropylene (PP), polyethylene terephthalate (PET), polystyrene (PS)], along with upcoming bioplastics polyhydroxyalkanoate (PHA) and polylactate (PLA) will be used as feedstock for microbial transformations. Consecutive controlled enzymatic and microbial degradation of mechanically pre-treated plastics wastes combined with subsequent microbial conversion to polymers and value-added chemicals by mixed cultures. Known plastic-degrading enzymes will be optimised by integrated protein engineering to achieve high specific binding capacities, stability, and catalytic efficacy towards a broad spectrum of plastic polymers under high salt and temperature conditions. Another focus lies in the search and isolation of novel enzymes active on recalcitrant polymers. MIX-UP will formulate enzyme cocktails tailored to specific waste streams and strives to enhance enzyme production significantly. In vivo and in vitro application of these cocktails enable stable, self-sustaining microbiomes to convert the released plastic monomers selectively into value-added products, key building blocks, and biomass. Any remaining material recalcitrant to the enzymatic activities will be recirculated into the process by physicochemical treatment. The Chinese-European MIX-UP consortium is multidisciplinary and industry-participating to address the market need for novel sustainable routes to valorise plastic waste streams. The project's new workflow realises a circular (bio)plastic economy and adds value to present poorly recycled plastic wastes where mechanical and chemical plastic recycling show limits.

Identifiants

pubmed: 34458054
doi: 10.1186/s12302-021-00536-5
pii: 536
pmc: PMC8380104
doi:

Types de publication

Journal Article

Langues

eng

Pagination

99

Informations de copyright

© The Author(s) 2021.

Déclaration de conflit d'intérêts

Competing interestsThe authors declare that they have no competing interests.

Références

Environ Sci Pollut Res Int. 2016 Jun;23(11):11349-11356
pubmed: 27072033
Adv Sci (Weinh). 2019 May 20;6(14):1900491
pubmed: 31380212
Environ Sci Technol. 2015 Oct 20;49(20):12080-6
pubmed: 26390034
Trends Biotechnol. 2021 Jan;39(1):12-23
pubmed: 32487438
Microb Biotechnol. 2017 Nov;10(6):1302-1307
pubmed: 28401691
Environ Sci Technol. 2015 Oct 20;49(20):12087-93
pubmed: 26390390
Sci Adv. 2017 Jul 19;3(7):e1700782
pubmed: 28776036
Sci Adv. 2020 Oct 30;6(44):
pubmed: 33127684
Appl Microbiol Biotechnol. 2019 Jan;103(1):143-157
pubmed: 30397765
Science. 2020 Jun 12;368(6496):1257-1260
pubmed: 32527833
Philos Trans R Soc Lond B Biol Sci. 2009 Jul 27;364(1526):1999-2012
pubmed: 19528052
Biotechnol Adv. 2013 Dec;31(8):1634-47
pubmed: 23978675
Proc Natl Acad Sci U S A. 2020 Oct 13;117(41):25476-25485
pubmed: 32989159
Bioresour Bioprocess. 2017;4(1):11
pubmed: 28251041
Science. 2017 Nov 17;358(6365):870-872
pubmed: 29146798
Microb Ecol. 2020 Apr;79(3):517-526
pubmed: 31463664
Appl Environ Microbiol. 1998 Apr;64(4):1366-71
pubmed: 9546174
Curr Opin Biotechnol. 2020 Apr;62:212-219
pubmed: 31881445
Sci Adv. 2020 Nov 20;6(47):
pubmed: 33219017
Chemosphere. 2017 Apr;173:520-528
pubmed: 28131922
Front Microbiol. 2020 Mar 17;11:382
pubmed: 32256468
Nat Commun. 2021 Mar 8;12(1):1513
pubmed: 33686068
ChemSusChem. 2020 Feb 7;13(3):488-492
pubmed: 31912617
Curr Opin Biotechnol. 2018 Apr;50:94-100
pubmed: 29223022
Polymers (Basel). 2017 Feb 16;9(2):
pubmed: 30970745
Microb Biotechnol. 2017 Nov;10(6):1308-1322
pubmed: 28371373
Nat Commun. 2020 Nov 13;11(1):5790
pubmed: 33188179
Metab Eng. 2020 Mar;58:82-93
pubmed: 31302223
Methods Enzymol. 2021;648:391-421
pubmed: 33579413
Science. 2020 Oct 23;370(6515):437-441
pubmed: 33093105
J Environ Manage. 2020 Jun 1;263:110402
pubmed: 32174537
Science. 2017 Feb 24;355(6327):814-816
pubmed: 28232574
Trends Biotechnol. 2021 Sep;39(9):953-963
pubmed: 33431229
Appl Environ Microbiol. 2014 Sep;80(17):5292-303
pubmed: 24951791
Methods Enzymol. 2021;648:159-185
pubmed: 33579402
Environ Pollut. 2021 Jan 15;269:116095
pubmed: 33257152
Environ Sci Technol. 2020 Oct 6;54(19):11657-11672
pubmed: 32886491
Science. 2020 Jun 5;368(6495):1140-1145
pubmed: 32354839
Environ Int. 2020 Dec;145:106106
pubmed: 32947161
Water Res. 2014 Jul 1;58:9-20
pubmed: 24731872
Bioprocess Biosyst Eng. 2014 Feb;37(2):225-33
pubmed: 23749235
Science. 2006 Dec 8;314(5805):1560-3
pubmed: 17158317
Science. 2017 Feb 24;355(6327):797-798
pubmed: 28232538
J Clin Invest. 2003 Nov;112(9):1291-9
pubmed: 14597753
Nature. 2020 Apr;580(7802):216-219
pubmed: 32269349
Microb Biotechnol. 2021 Mar;14(2):374-385
pubmed: 32343496
Waste Manag. 2019 Feb 15;85:141-150
pubmed: 30803567
Sci Adv. 2018 Aug 10;4(8):eaat9669
pubmed: 30105308
Chemosphere. 2018 Jan;191:979-989
pubmed: 29145143
Science. 2016 Mar 11;351(6278):1196-9
pubmed: 26965627
Microb Biotechnol. 2015 Nov;8(6):900-3
pubmed: 26482561
Science. 2020 Sep 18;369(6510):1515-1518
pubmed: 32943526
Environ Sci Technol. 2019 May 7;53(9):5256-5265
pubmed: 30990998
Biotechnol Adv. 2020 Mar - Apr;39:107457
pubmed: 31689471
Science. 2020 Oct 23;370(6515):400-401
pubmed: 33093094
Environ Sci Technol. 2020 Jun 2;54(11):6987-6996
pubmed: 32374590
Methods Enzymol. 2021;648:95-120
pubmed: 33579419
Appl Microbiol Biotechnol. 2015 Nov;99(21):8857-74
pubmed: 26318446
Biotechnol Biofuels. 2015 Jan 23;8(1):10
pubmed: 25648981
Mol Syst Biol. 2007;3:92
pubmed: 17353934
Metab Eng. 2021 Jul;66:167-178
pubmed: 33865980
Macromol Biosci. 2006 Nov 9;6(11):885-906
pubmed: 17099863

Auteurs

Hendrik Ballerstedt (H)

Institute of Applied Microbiology (iAMB), Aachen Biology and Biotechnology (ABBt), RWTH Aachen University, Worringerweg 1, 52074 Aachen, Germany.

Till Tiso (T)

Institute of Applied Microbiology (iAMB), Aachen Biology and Biotechnology (ABBt), RWTH Aachen University, Worringerweg 1, 52074 Aachen, Germany.

Nick Wierckx (N)

Institute of Bio- and Geosciences IBG-1: Biotechnology, Research Center Jülich, Wilhelm Johnen Straße, 52428 Jülich, Germany.

Ren Wei (R)

Institute of Biochemistry, University of Greifswald, Felix-Hausdorff-Str. 4, 17487 Greifswald, Germany.

Luc Averous (L)

BioTeam/ICPEES-ECPM, UMR CNRS 7515, Université de Strasbourg, 25 rue Becquerel, 67087 Strasbourg Cedex 2, France.

Uwe Bornscheuer (U)

Institute of Biochemistry, University of Greifswald, Felix-Hausdorff-Str. 4, 17487 Greifswald, Germany.

Kevin O'Connor (K)

BiOrbic Bioeconomy SFI Research Centre, UCD Earth Institute and School of Biomolecular and Biomedical Science, University College Dublin, Belfield, Dublin 4, Ireland.

Tilman Floehr (T)

everwave GmbH, Strüverweg 116, 52070 Aachen, Germany.

Andreas Jupke (A)

Fluid Process Engineering, Aachen Process Technology (AVT), RWTH Aachen University, Forckenbeckstraße 51, 52074 Aachen, Germany.

Jürgen Klankermayer (J)

Institute of Technical and Macromolecular Chemistry (ITMC), RWTH Aachen University, Worringerweg 2, 52074 Aachen, Germany.

Luo Liu (L)

College of Life Science and Technology (CLST), Beijing University of Chemical Technology, Beisanhuan EastRoad 15, Chaoyang District, Beijing, 100029 PR China.

Victor de Lorenzo (V)

Interdisciplinary Platform for Sustainable Plastics Towards a Circular Economy-Spanish National Research Council (SusPlast-CSIC), Biological Research Center (CIB-CSIC), 28040 Madrid, Spain.

Tanja Narancic (T)

BiOrbic Bioeconomy SFI Research Centre, UCD Earth Institute and School of Biomolecular and Biomedical Science, University College Dublin, Belfield, Dublin 4, Ireland.

Juan Nogales (J)

Interdisciplinary Platform for Sustainable Plastics Towards a Circular Economy-Spanish National Research Council (SusPlast-CSIC), Biological Research Center (CIB-CSIC), 28040 Madrid, Spain.

Rémi Perrin (R)

SOPREMA, Direction R&D, 14 Rue Saint Nazaire, 67100 Strasbourg, France.

Eric Pollet (E)

BioTeam/ICPEES-ECPM, UMR CNRS 7515, Université de Strasbourg, 25 rue Becquerel, 67087 Strasbourg Cedex 2, France.

Auxiliadora Prieto (A)

Interdisciplinary Platform for Sustainable Plastics Towards a Circular Economy-Spanish National Research Council (SusPlast-CSIC), Biological Research Center (CIB-CSIC), 28040 Madrid, Spain.

William Casey (W)

Bioplastech Ltd., Nova UCD, Belfield Innovation Park, University College Dublin, Belfield, Dublin 4, Ireland.

Thomas Haarmann (T)

AB Enzymes GmbH, Feldbergstraße 78, 64293 Darmstadt, Germany.

Alexandru Sarbu (A)

SOPREMA, Direction R&D, 14 Rue Saint Nazaire, 67100 Strasbourg, France.

Ulrich Schwaneberg (U)

Institute of Biotechnology (BIOTEC), Aachen Biology and Biotechnology (ABBt), RWTH Aachen University, Worringerweg 3, 52074 Aachen, Germany.

Fengxue Xin (F)

College of Biotechnology and Pharmaceutical Engineering, Nanjing Tech University, No. 30 Puzhu Road, Nanjing, 211816 PR China.

Weiliang Dong (W)

College of Biotechnology and Pharmaceutical Engineering, Nanjing Tech University, No. 30 Puzhu Road, Nanjing, 211816 PR China.

Jiamin Xing (J)

State Key Laboratory of Biochemical Engineering, Institute of Process Engineering (IPE), Chinese Academy of Sciences, 1 North 2nd Street, Zhongguancun, Beijing, 100190 PR China.

Guo-Qiang Chen (GQ)

School of Life Sciences (SLS), Tsinghua University, Beijing, 100084 PR China.

Tianwei Tan (T)

College of Life Science and Technology (CLST), Beijing University of Chemical Technology, Beisanhuan EastRoad 15, Chaoyang District, Beijing, 100029 PR China.

Min Jiang (M)

College of Biotechnology and Pharmaceutical Engineering, Nanjing Tech University, No. 30 Puzhu Road, Nanjing, 211816 PR China.

Lars M Blank (LM)

Institute of Applied Microbiology (iAMB), Aachen Biology and Biotechnology (ABBt), RWTH Aachen University, Worringerweg 1, 52074 Aachen, Germany.

Classifications MeSH