Single-Junction Organic Photovoltaic Cell with 19% Efficiency.
energy loss
light utilization
molecular design
organic photovoltaic cells
power conversion efficiency
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Oct 2021
Oct 2021
Historique:
revised:
24
05
2021
received:
29
03
2021
pubmed:
1
9
2021
medline:
1
9
2021
entrez:
31
8
2021
Statut:
ppublish
Résumé
Improving power conversion efficiency (PCE) is important for broadening the applications of organic photovoltaic (OPV) cells. Here, a maximum PCE of 19.0% (certified value of 18.7%) is achieved in single-junction OPV cells by combining material design with a ternary blending strategy. An active layer comprising a new wide-bandgap polymer donor named PBQx-TF and a new low-bandgap non-fullerene acceptor (NFA) named eC9-2Cl is rationally designed. With optimized light utilization, the resulting binary cell exhibits a good PCE of 17.7%. An NFA F-BTA3 is then added to the active layer as a third component to simultaneously improve the photovoltaic parameters. The improved light unitization, cascaded energy level alignment, and enhanced intermolecular packing result in open-circuit voltage of 0.879 V, short-circuit current density of 26.7 mA cm
Identifiants
pubmed: 34464466
doi: 10.1002/adma.202102420
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2102420Subventions
Organisme : National Key Research and Development Program of China
ID : 2019YFA0705901
Organisme : MOST and the Basic and Applied Basic Research Major Program of Guangdong Province
ID : 2019B030302007
Organisme : National Natural Science Foundation of China
ID : 52003275
Organisme : National Natural Science Foundation of China
ID : 51961135103
Organisme : National Natural Science Foundation of China
ID : 21805287
Organisme : National Natural Science Foundation of China
ID : 22075301
Organisme : National Natural Science Foundation of China
ID : 21734008
Organisme : Youth Innovation Promotion Association
Organisme : China Postdoctoral Science Foundation
ID : 2019M660800
Organisme : China Postdoctoral Science Foundation
ID : 2019M660799
Organisme : Beijing National Laboratory for Molecular Sciences
ID : BNLMS-CXXM-201903
Organisme : Beijing National Laboratory for Molecular Sciences
ID : 2019BMS20005
Organisme : Youth Innovation Promotion Association of the Chinese Academy of Sciences
ID : 2018043
Informations de copyright
© 2021 Wiley-VCH GmbH.
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