Ultrafast and long-time excited state kinetics of an NIR-emissive vanadium(iii) complex I: synthesis, spectroscopy and static quantum chemistry.


Journal

Chemical science
ISSN: 2041-6520
Titre abrégé: Chem Sci
Pays: England
ID NLM: 101545951

Informations de publication

Date de publication:
18 Aug 2021
Historique:
received: 16 04 2021
accepted: 07 07 2021
entrez: 3 9 2021
pubmed: 4 9 2021
medline: 4 9 2021
Statut: epublish

Résumé

In spite of intense, recent research efforts, luminescent transition metal complexes with Earth-abundant metals are still very rare owing to the small ligand field splitting of 3d transition metal complexes and the resulting non-emissive low-energy metal-centered states. Low-energy excited states decay efficiently non-radiatively, so that near-infrared emissive transition metal complexes with 3d transition metals are even more challenging. We report that the heteroleptic pseudo-octahedral d

Identifiants

pubmed: 34476059
doi: 10.1039/d1sc02137k
pii: d1sc02137k
pmc: PMC8372323
doi:

Types de publication

Journal Article

Langues

eng

Pagination

10780-10790

Informations de copyright

This journal is © The Royal Society of Chemistry.

Déclaration de conflit d'intérêts

There are no conflicts to declare.

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Auteurs

Matthias Dorn (M)

Department of Chemistry, Johannes Gutenberg University of Mainz Duesbergweg 10-14 55128 Mainz Germany katja.heinze@uni-mainz.de.

Jens Kalmbach (J)

Institute of Inorganic Chemistry, University of Tübingen Auf der Morgenstelle 18 72076 Tübingen Germany.

Pit Boden (P)

Department of Chemistry and Research Center Optimas, Technical University Kaiserslautern Erwin-Schrödinger-Straße 67663 Kaiserslautern Germany.

Ayla Kruse (A)

Institute for Physics, Department of Life, Light and Matter, University of Rostock 18051 Rostock Germany.

Chahinez Dab (C)

Département de chimie, Université de Montréal Montréal Québec H3C 3J7 Canada.

Christian Reber (C)

Département de chimie, Université de Montréal Montréal Québec H3C 3J7 Canada.

Gereon Niedner-Schatteburg (G)

Department of Chemistry and Research Center Optimas, Technical University Kaiserslautern Erwin-Schrödinger-Straße 67663 Kaiserslautern Germany.

Stefan Lochbrunner (S)

Institute for Physics, Department of Life, Light and Matter, University of Rostock 18051 Rostock Germany.

Markus Gerhards (M)

Department of Chemistry and Research Center Optimas, Technical University Kaiserslautern Erwin-Schrödinger-Straße 67663 Kaiserslautern Germany.

Michael Seitz (M)

Institute of Inorganic Chemistry, University of Tübingen Auf der Morgenstelle 18 72076 Tübingen Germany.

Katja Heinze (K)

Department of Chemistry, Johannes Gutenberg University of Mainz Duesbergweg 10-14 55128 Mainz Germany katja.heinze@uni-mainz.de.

Classifications MeSH