Design of a Zn Single-Site Curing Activator for a More Sustainable Sulfur Cross-Link Formation in Rubber.


Journal

Industrial & engineering chemistry research
ISSN: 0888-5885
Titre abrégé: Ind Eng Chem Res
Pays: United States
ID NLM: 9882836

Informations de publication

Date de publication:
21 Jul 2021
Historique:
received: 26 04 2021
revised: 23 06 2021
accepted: 24 06 2021
entrez: 6 9 2021
pubmed: 7 9 2021
medline: 7 9 2021
Statut: ppublish

Résumé

ZnO is a worldwide used activator for a rubber vulcanization process, which promotes fast curing kinetics and high cross-linking densities of rubber nanocomposites (NCs). However, its extended use together with leaching phenomena occurring during the production and life cycle of rubber products, especially tires, entails potential environmental risks, as ecotoxicity toward aquatic organisms. Pushed by this issue, a novel activator was developed, which introduces highly dispersed and active zinc species in the vulcanization process, reducing the amount of employed ZnO and keeping high the curing efficiency. The activator is constituted by Zn(II) single sites, anchored on the surface of SiO

Identifiants

pubmed: 34483477
doi: 10.1021/acs.iecr.1c01580
pmc: PMC8411846
doi:

Types de publication

Journal Article

Langues

eng

Pagination

10180-10192

Informations de copyright

© 2021 The Authors. Published by American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

Références

Materials (Basel). 2014 Apr 09;7(4):2833-2881
pubmed: 28788596
Nanoscale. 2020 Dec 23;12(48):24527-24542
pubmed: 33320147
Waste Manag. 2013 Mar;33(3):679-88
pubmed: 23063305
Environ Sci Technol. 2004 Aug 1;38(15):4206-14
pubmed: 15352462
Arch Biochem Biophys. 1974 Dec;165(2):691-708
pubmed: 4374138
Environ Sci Technol. 2006 Jul 15;40(14):4374-81
pubmed: 16903273
Environ Pollut. 2013 Jan;172:76-85
pubmed: 22995930
Phys Chem Chem Phys. 2010 Mar 28;12(12):3014-30
pubmed: 20449394
Environ Toxicol Chem. 2014 Jan;33(1):190-8
pubmed: 24123301
Integr Environ Assess Manag. 2005 Nov;1(4):301-19
pubmed: 16639898
J Am Chem Soc. 2017 Jan 11;139(1):389-408
pubmed: 27951638
Ecotoxicol Environ Saf. 2015 Mar;113:23-30
pubmed: 25483368
Chemosphere. 2011 Oct;85(5):738-43
pubmed: 21737116
Sci Total Environ. 2010 Sep 15;408(20):4271-84
pubmed: 20619879
Phys Chem Chem Phys. 2017 May 31;19(21):14114-14128
pubmed: 28524206

Auteurs

Silvia Mostoni (S)

Department of Materials Science, INSTM, University of Milano-Bicocca, Via R. Cozzi 55, Milano 20125, Italy.

Massimiliano D'Arienzo (M)

Department of Materials Science, INSTM, University of Milano-Bicocca, Via R. Cozzi 55, Milano 20125, Italy.

Barbara Di Credico (B)

Department of Materials Science, INSTM, University of Milano-Bicocca, Via R. Cozzi 55, Milano 20125, Italy.

Lidia Armelao (L)

Institute of Condensed Matter Chemistry and Technologies for Energy, National Research Council of Italy, ICMATE-CNR, via Marzolo 1, Padua 35131, Italy.
Department of Chemical Sciences, University of Padua, Via Marzolo 1, Padua 35131, Italy.
Department of Chemical Sciences and Materials Technologies, National Research Council of Italy, DSCTM-CNR, Piazzale A. Moro 7, Rome 00185, Italy.

Marzio Rancan (M)

Institute of Condensed Matter Chemistry and Technologies for Energy, National Research Council of Italy, ICMATE-CNR, via Marzolo 1, Padua 35131, Italy.

Sandra Dirè (S)

"Klaus Müller" Magnetic Resonance Lab., Dept. of Industrial Engineering, University of Trento, Via Sommarive 9, Trento 38123, Italy.

Emanuela Callone (E)

"Klaus Müller" Magnetic Resonance Lab., Dept. of Industrial Engineering, University of Trento, Via Sommarive 9, Trento 38123, Italy.

Raffaella Donetti (R)

Pirelli Tyre SpA, Viale Sarca 222, Milano 20126, Italy.

Antonio Susanna (A)

Pirelli Tyre SpA, Viale Sarca 222, Milano 20126, Italy.

Roberto Scotti (R)

Department of Materials Science, INSTM, University of Milano-Bicocca, Via R. Cozzi 55, Milano 20125, Italy.

Classifications MeSH