Current pollution status, spatial features, and health risks of legacy and emerging halogenated flame retardants in agricultural soils across China.

Soil is a major reservoir and a secondary source of semi-volatile organic chemicals, while studies on the pollution status of halogenated flame retardants (HFRs) in agricultural soils are limited. In this study, a total of twenty-five chemicals including novel brominated flame retardants (NBFRs), polybrominated diphenyl ethers (PBDEs), and dechlorane plus (DPs) was analyzed in the agricultural soils across China to investigate the occurrence, spatial distribution, potential sources, influencing factors and their associated human health risks. The results showed that BDE-209 (125-130,183 pg/g, dry weight, d.w.) was the most abundant flame retardant of PBDEs, followed by decabromodiphenyl ethane (DBDPE) (9.27-22,864 pg/g, d.w.). Meanwhile, the DPs (anti-DP plus syn-DP) were in the range of ND-1229 pg/g (d.w.), and the range of f

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Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.