Fluorophore-PNA-Quencher/Quencher-DNA probe for miRNA detection.


Journal

Bioorganic & medicinal chemistry letters
ISSN: 1464-3405
Titre abrégé: Bioorg Med Chem Lett
Pays: England
ID NLM: 9107377

Informations de publication

Date de publication:
01 11 2021
Historique:
received: 06 07 2021
revised: 26 08 2021
accepted: 09 09 2021
pubmed: 18 9 2021
medline: 11 1 2022
entrez: 17 9 2021
Statut: ppublish

Résumé

Micro RNAs (miRNAs) are involved in a variety of biological functions and are attracting attention as diagnostic and prognostic markers for various diseases. Highly sensitive RNA detection methods are required to determine miRNA expression levels and intracellular localization. In this study, we designed new double-stranded peptide nucleic acid (PNA)/DNA probes consisting of a fluorophore-PNA-quencher (fPq) and a quencher-DNA (qD) for miR-221 detection. We optimized the fPq structure, PNA-DNA hybrid length, and hybrid position. The resultant fPq-2/qD-6b probe was a 6-bp hybrid probe with a 10-base fPq and a 6-base qD. The signal-to-background ratios of the probes showed that fPq-2/qD-6b had a higher target sensitivity than fPq (PNA beacon)-type and fP/qD-type probes. The results of the detection limit and target specificity indicate that the fPq/qD probe is promising for RNA detection in both cells and cell extracts as well as for miRNA diagnosis.

Identifiants

pubmed: 34534675
pii: S0960-894X(21)00586-2
doi: 10.1016/j.bmcl.2021.128359
pii:
doi:

Substances chimiques

DNA Probes 0
Fluorescent Dyes 0
MicroRNAs 0
Peptide Nucleic Acids 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

128359

Informations de copyright

Copyright © 2021 Elsevier Ltd. All rights reserved.

Auteurs

Kentaro Tabara (K)

Department of Interdisciplinary Science and Engineering in Health Systems, Okayama University, Okayama, Japan.

Kazunori Watanabe (K)

Department of Interdisciplinary Science and Engineering in Health Systems, Okayama University, Okayama, Japan.

Hajime Shigeto (H)

Health and Medical Research Institute, National Institute of Advanced Industrial Science and Technology, 2217-14 Hayashi-cho, Takamatsu, Kagawa 761-0395, Japan.

Shohei Yamamura (S)

Health and Medical Research Institute, National Institute of Advanced Industrial Science and Technology, 2217-14 Hayashi-cho, Takamatsu, Kagawa 761-0395, Japan.

Takamasa Kishi (T)

Department of Applied Chemistry, Kindai University, 3-4-1 Kowakae, Higashi-Osaka, Osaka 577-8502, Japan.

Mizuki Kitamatsu (M)

Department of Applied Chemistry, Kindai University, 3-4-1 Kowakae, Higashi-Osaka, Osaka 577-8502, Japan.

Takashi Ohtsuki (T)

Department of Interdisciplinary Science and Engineering in Health Systems, Okayama University, Okayama, Japan. Electronic address: ohtsuk@okayama-u.ac.jp.

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Classifications MeSH