Heterogeneous Functional Dielectric Patterns for Charge-Carrier Modulation in Ultraflexible Organic Integrated Circuits.
charge-carrier modulation
flexible electronics
functional dielectric patterns
integrated circuits
organic transistors
polymer dielectrics
threshold voltage control
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Nov 2021
Nov 2021
Historique:
revised:
11
08
2021
received:
10
06
2021
pubmed:
22
9
2021
medline:
22
9
2021
entrez:
21
9
2021
Statut:
ppublish
Résumé
Flexible electronics have gained considerable attention for application in wearable devices. Organic transistors are potential candidates to develop flexible integrated circuits (ICs). A primary technique for maximizing their reliability, gain, and operation speed is the modulation of charge-carrier behavior in the respective transistors fabricated on the same substrate. In this work, heterogeneous functional dielectric patterns (HFDP) of ultrathin polymer gate dielectrics of poly((±)endo,exo-bicyclo[2.2.1]hept-ene-2,3-dicarboxylic acid, diphenylester) (PNDPE) are introduced. The HFDP that are obtained via the photo-Fries rearrangement by ultraviolet radiation in the homogeneous PNDPE provide a functional area for charge-carrier modulation. This leads to programmable threshold voltage control over a wide range (-1.5 to +0.2 V) in the transistors with a high patterning resolution, at 2 V operational voltage. The transistors also exhibit high operational stability over 140 days and under the bias-stress duration of 1800 s. With the HFDP, the performance metrics of ICs, for example, the noise margin and gain of the zero-V
Identifiants
pubmed: 34545628
doi: 10.1002/adma.202104446
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2104446Subventions
Organisme : Ministry of Education, Culture, Sports, Science and Technology
ID : JPMXP09F20OS0045
Organisme : Ministry of Education, Culture, Sports, Science and Technology
ID : JPMXP09S20OS0019
Organisme : Advanced Photonics and Biosensing Open Innovation Laboratory
Organisme : National Institute of Advanced Industrial Science and Technology
Organisme : Japan Science and Technology Agency
ID : JPMJFR2035
Organisme : Japan Science and Technology Agency
ID : JPMJFR2022
Organisme : Japan Society for the Promotion of Science
ID : 19H01174
Organisme : Japan Society for the Promotion of Science
ID : 20K21003
Organisme : Japan Society for the Promotion of Science
ID : 18H01861
Organisme : Japan Society for the Promotion of Science
ID : 19H02199
Informations de copyright
© 2021 The Authors. Advanced Materials published by Wiley-VCH GmbH.
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