Significance of the organic aerosol driven climate feedback in the boreal area.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
24 09 2021
Historique:
received: 23 03 2021
accepted: 01 09 2021
entrez: 25 9 2021
pubmed: 26 9 2021
medline: 26 9 2021
Statut: epublish

Résumé

Aerosol particles cool the climate by scattering solar radiation and by acting as cloud condensation nuclei. Higher temperatures resulting from increased greenhouse gas levels have been suggested to lead to increased biogenic secondary organic aerosol and cloud condensation nuclei concentrations creating a negative climate feedback mechanism. Here, we present direct observations on this feedback mechanism utilizing collocated long term aerosol chemical composition measurements and remote sensing observations on aerosol and cloud properties. Summer time organic aerosol loadings showed a clear increase with temperature, with simultaneous increase in cloud condensation nuclei concentration in a boreal forest environment. Remote sensing observations revealed a change in cloud properties with an increase in cloud reflectivity in concert with increasing organic aerosol loadings in the area. The results provide direct observational evidence on the significance of this negative climate feedback mechanism.

Identifiants

pubmed: 34561456
doi: 10.1038/s41467-021-25850-7
pii: 10.1038/s41467-021-25850-7
pmc: PMC8463617
doi:

Types de publication

Journal Article Research Support, U.S. Gov't, Non-P.H.S. Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

5637

Informations de copyright

© 2021. The Author(s).

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Auteurs

Taina Yli-Juuti (T)

Department of Applied Physics, University of Eastern Finland, Kuopio, Finland. taina.yli-juuti@uef.fi.

Tero Mielonen (T)

Atmospheric Research Centre of Eastern Finland, Finnish Meteorological Institute, Kuopio, Finland.

Liine Heikkinen (L)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland.

Antti Arola (A)

Atmospheric Research Centre of Eastern Finland, Finnish Meteorological Institute, Kuopio, Finland.

Mikael Ehn (M)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland.

Sini Isokääntä (S)

Department of Applied Physics, University of Eastern Finland, Kuopio, Finland.

Helmi-Marja Keskinen (HM)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland.
Aerosol Physics Laboratory, Physics Unit, Tampere University, Tampere, Finland.

Markku Kulmala (M)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland.

Anton Laakso (A)

Atmospheric Research Centre of Eastern Finland, Finnish Meteorological Institute, Kuopio, Finland.

Antti Lipponen (A)

Atmospheric Research Centre of Eastern Finland, Finnish Meteorological Institute, Kuopio, Finland.

Krista Luoma (K)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland.

Santtu Mikkonen (S)

Department of Applied Physics, University of Eastern Finland, Kuopio, Finland.
Department of Environmental and Biological Sciences, University of Eastern Finland, Kuopio, Finland.

Tuomo Nieminen (T)

Department of Applied Physics, University of Eastern Finland, Kuopio, Finland.
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland.
Institute for Atmospheric and Earth System Research/Forest Sciences, Faculty of Agriculture and Forestry, University of Helsinki, Helsinki, Finland.

Pauli Paasonen (P)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland.

Tuukka Petäjä (T)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland.

Sami Romakkaniemi (S)

Atmospheric Research Centre of Eastern Finland, Finnish Meteorological Institute, Kuopio, Finland.

Juha Tonttila (J)

Atmospheric Research Centre of Eastern Finland, Finnish Meteorological Institute, Kuopio, Finland.

Harri Kokkola (H)

Atmospheric Research Centre of Eastern Finland, Finnish Meteorological Institute, Kuopio, Finland.

Annele Virtanen (A)

Department of Applied Physics, University of Eastern Finland, Kuopio, Finland.

Classifications MeSH