Photo-Thermal Switching of Individual Plasmonically Activated Spin Crossover Nanoparticle Imaged by Ultrafast Transmission Electron Microscopy.
nanohybrids
single nanoparticle detection
spin crossover
time-resolved spectroscopy
ultrafast electron microscopy
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Dec 2021
Dec 2021
Historique:
revised:
22
09
2021
received:
19
07
2021
pubmed:
4
10
2021
medline:
4
10
2021
entrez:
3
10
2021
Statut:
ppublish
Résumé
Spin crossover (SCO) is a promising switching phenomenon when implemented in electronic devices as molecules, thin films or nanoparticles. Among the properties modulated along this phenomenon, optically induced mechanical changes are of tremendous importance as they can work as fast light-induced mechanical switches or allow to investigate and control microstructural strains and fatigability. The development of characterization techniques probing nanoscopic behavior with high spatio-temporal resolution allows to trigger and visualize such mechanical changes of individual nanoscopic objects. Here, ultrafast transmission electron microscopy (UTEM) is used to precisely probe the length changes of individual switchable nanoparticles induced thermally by nanosecond laser pulses. This allows revealing of the mechanisms of spin switching, leading to the macroscopic expansion of SCO materials. This study is conducted on individual pure SCO nanoparticles and SCO nanoparticles encapsulating gold nanorods that serve for plasmonic heating under laser pulses. Length changes are compared with time-resolved optical measurements performed on an assembly of these particles.
Identifiants
pubmed: 34601766
doi: 10.1002/adma.202105586
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2105586Subventions
Organisme : CNRS
Organisme : Nouvelle Aquitaine Region
Organisme : ANR
ID : ANR-17-CE09-0010-01
Organisme : Agence Nationale de Recherche
ID : ANR-11-EQPX-0041
Organisme : China Scholarship Council
Organisme : Agence Nationale de la Recherche
ID : ANR-11-EQPX-0041
Informations de copyright
© 2021 Wiley-VCH GmbH.
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