Fröhlich interaction dominated by a single phonon mode in CsPbBr


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
06 Oct 2021
Historique:
received: 11 01 2021
accepted: 17 09 2021
entrez: 7 10 2021
pubmed: 8 10 2021
medline: 8 10 2021
Statut: epublish

Résumé

The excellent optoelectronic performance of lead halide perovskites has generated great interest in their fundamental properties. The polar nature of the perovskite lattice means that electron-lattice coupling is governed by the Fröhlich interaction. Still, considerable ambiguity exists regarding the phonon modes that participate in this crucial mechanism. Here, we use multiphonon Raman scattering and THz time-domain spectroscopy to investigate Fröhlich coupling in CsPbBr

Identifiants

pubmed: 34615880
doi: 10.1038/s41467-021-26192-0
pii: 10.1038/s41467-021-26192-0
pmc: PMC8494801
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

5844

Subventions

Organisme : Nederlandse Organisatie voor Wetenschappelijk Onderzoek (Netherlands Organisation for Scientific Research)
ID : DDC13
Organisme : Nederlandse Organisatie voor Wetenschappelijk Onderzoek (Netherlands Organisation for Scientific Research)
ID : DDC13
Organisme : Nederlandse Organisatie voor Wetenschappelijk Onderzoek (Netherlands Organisation for Scientific Research)
ID : DDC13

Informations de copyright

© 2021. The Author(s).

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Auteurs

Claudiu M Iaru (CM)

Department of Applied Physics and Institute for Photonic Integration, Eindhoven University of Technology, P.O. Box 513, 5600 MB, Eindhoven, The Netherlands. C.M.Iaru@tue.nl.

Annalisa Brodu (A)

Condensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht University, Princetonplein 1, 3508 TA, Utrecht, The Netherlands.

Niels J J van Hoof (NJJ)

Department of Applied Physics and Institute for Photonic Integration, Eindhoven University of Technology, P.O. Box 513, 5600 MB, Eindhoven, The Netherlands.

Stan E T Ter Huurne (SET)

Department of Applied Physics and Institute for Photonic Integration, Eindhoven University of Technology, P.O. Box 513, 5600 MB, Eindhoven, The Netherlands.

Jonathan Buhot (J)

HH Wills Laboratory, University of Bristol, Bristol, BS8 1TL, UK.
High Field Magnet Laboratory (HFML - EMFL), Radboud University, 6525 ED, Nijmegen, The Netherlands.

Federico Montanarella (F)

Condensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht University, Princetonplein 1, 3508 TA, Utrecht, The Netherlands.

Sophia Buhbut (S)

Condensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht University, Princetonplein 1, 3508 TA, Utrecht, The Netherlands.

Peter C M Christianen (PCM)

High Field Magnet Laboratory (HFML - EMFL), Radboud University, 6525 ED, Nijmegen, The Netherlands.

Daniël Vanmaekelbergh (D)

Condensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht University, Princetonplein 1, 3508 TA, Utrecht, The Netherlands.

Celso de Mello Donega (C)

Condensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht University, Princetonplein 1, 3508 TA, Utrecht, The Netherlands.

Jaime Gòmez Rivas (JG)

Department of Applied Physics and Institute for Photonic Integration, Eindhoven University of Technology, P.O. Box 513, 5600 MB, Eindhoven, The Netherlands.

Paul M Koenraad (PM)

Department of Applied Physics and Institute for Photonic Integration, Eindhoven University of Technology, P.O. Box 513, 5600 MB, Eindhoven, The Netherlands.

Andrei Yu Silov (AY)

Department of Applied Physics and Institute for Photonic Integration, Eindhoven University of Technology, P.O. Box 513, 5600 MB, Eindhoven, The Netherlands. A.Y.Silov@tue.nl.

Classifications MeSH