Facile Synthesis of Palladium-Based Nanocrystals with Different Crystal Phases and a Comparison of Their Catalytic Properties.
catalysis
nanocrystals
palladium
phase-control
ruthenium
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Dec 2021
Dec 2021
Historique:
revised:
12
09
2021
received:
20
05
2021
pubmed:
9
10
2021
medline:
9
10
2021
entrez:
8
10
2021
Statut:
ppublish
Résumé
A relatively unexplored aspect of noble-metal nanomaterials is polymorphism, or their ability to crystallize in different crystal phases. Here, a method is reported for the facile synthesis of Ru@Pd core-shell nanocrystals featuring polymorphism, with the core made of hexagonally close-packed (hcp)-Ru while the Pd shell takes either an hcp or face-centered cubic (fcc) phase. The polymorphism shows a dependence on the shell thickness, with shells thinner than ≈1.4 nm taking the hcp phase whereas the thicker ones revert to fcc. The injection rate provides an experimental knob for controlling the phase, with one-shot and drop-wise injection of the Pd precursor corresponding to fcc-Pd and hcp-Pd shells, respectively. When these nanocrystals are tested as catalysts toward formic acid oxidation, the Ru@Pd
Identifiants
pubmed: 34623694
doi: 10.1002/adma.202103801
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2103801Subventions
Organisme : NSF
ID : CHE 1804970
Organisme : National Science Foundation
ID : ECCS-1542174
Organisme : National Energy Research Scientific Computing Center
Organisme : DOE Office of Science User Facility located at Lawrence Berkeley National Laboratory and operated
ID : DE-AC02-05CH11231
Informations de copyright
© 2021 Wiley-VCH GmbH.
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