Roles of Organic Fragments in Redirecting Crystal/Molecular Structures of Inorganic-Organic Hybrids Based on Lacunary Keggin-Type Polyoxometalates.
Keggin
inorganic–organic hybrids
lacunary
polyoxometalates
rare earth
Journal
Molecules (Basel, Switzerland)
ISSN: 1420-3049
Titre abrégé: Molecules
Pays: Switzerland
ID NLM: 100964009
Informations de publication
Date de publication:
02 Oct 2021
02 Oct 2021
Historique:
received:
26
08
2021
revised:
25
09
2021
accepted:
29
09
2021
entrez:
13
10
2021
pubmed:
14
10
2021
medline:
14
10
2021
Statut:
epublish
Résumé
Lacunary polyoxometalates (LPOMs) are key precursors for the synthesis of functional POMs. To date, reviews dedicated to behavioral studies of LPOMs often comprise the role of metal ions, including transition metal (TM) and rare earth (RE) ions, in extending and stability of high-nuclearity clusters. In contrast, the role of organic ligands in the structures and properties of lacunary-based hybrids has remained less explored. In this review, we focus on the role of organic fragments in the self-assembling process of POM-based architectures and discuss relationships between the nature and structure of organic ligand and properties such as the topology of hybrid inorganic-organic material in RE and TM-RE heterometallic derivatives of lacunary Keggin-type POMs. The effects of organic fragment in mixed ligand hybrids are also briefly reviewed.
Identifiants
pubmed: 34641537
pii: molecules26195994
doi: 10.3390/molecules26195994
pmc: PMC8512714
pii:
doi:
Types de publication
Journal Article
Review
Langues
eng
Sous-ensembles de citation
IM
Subventions
Organisme : Ferdowsi University of Mashhad
ID : 3/35582
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