Overcoming the Rate-Directionality Trade-off: A Room-Temperature Ultrabright Quantum Light Source.
Purcell factor
colloidal nanocrystals
directional emission
nanoantenna
plasmonic resonator
quantum dots
single-photon source
Journal
ACS nano
ISSN: 1936-086X
Titre abrégé: ACS Nano
Pays: United States
ID NLM: 101313589
Informations de publication
Date de publication:
23 Nov 2021
23 Nov 2021
Historique:
pubmed:
20
10
2021
medline:
20
10
2021
entrez:
19
10
2021
Statut:
ppublish
Résumé
Deterministic GHz-rate single photon sources at room temperature would be essential components for various quantum applications. However, both the slow intrinsic decay rate and the omnidirectional emission of typical quantum emitters are two obstacles toward achieving such a goal which are hard to overcome simultaneously. Here, we solve this challenge by a hybrid approach using a complex monolithic photonic resonator constructed of a gold nanocone responsible for the rate enhancement, enclosed by a circular Bragg antenna for emission directionality. A repeatable process accurately binds quantum dots to the tip of the antenna-embedded nanocone. As a result, we achieve simultaneous 20-fold emission rate enhancement and record-high directionality leading to an increase in the observed brightness by a factor as large as 800 (130) into an NA = 0.22(0.5). We project that these miniaturized on-chip devices can reach photon rates approaching 1.4 × 10
Identifiants
pubmed: 34664938
doi: 10.1021/acsnano.1c08591
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM