Overcoming the Rate-Directionality Trade-off: A Room-Temperature Ultrabright Quantum Light Source.

Purcell factor colloidal nanocrystals directional emission nanoantenna plasmonic resonator quantum dots single-photon source

Journal

ACS nano
ISSN: 1936-086X
Titre abrégé: ACS Nano
Pays: United States
ID NLM: 101313589

Informations de publication

Date de publication:
23 Nov 2021
Historique:
pubmed: 20 10 2021
medline: 20 10 2021
entrez: 19 10 2021
Statut: ppublish

Résumé

Deterministic GHz-rate single photon sources at room temperature would be essential components for various quantum applications. However, both the slow intrinsic decay rate and the omnidirectional emission of typical quantum emitters are two obstacles toward achieving such a goal which are hard to overcome simultaneously. Here, we solve this challenge by a hybrid approach using a complex monolithic photonic resonator constructed of a gold nanocone responsible for the rate enhancement, enclosed by a circular Bragg antenna for emission directionality. A repeatable process accurately binds quantum dots to the tip of the antenna-embedded nanocone. As a result, we achieve simultaneous 20-fold emission rate enhancement and record-high directionality leading to an increase in the observed brightness by a factor as large as 800 (130) into an NA = 0.22(0.5). We project that these miniaturized on-chip devices can reach photon rates approaching 1.4 × 10

Identifiants

pubmed: 34664938
doi: 10.1021/acsnano.1c08591
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

17384-17391

Auteurs

Hamza Abudayyeh (H)

Racah Institute of Physics, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.
The Center for Nanoscience and Nanotechnology, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.

Annika Mildner (A)

Institute for Applied Physics and Center LISA+, University of Tuebingen, Auf der Morgenstelle 10, 72076, Tuebingen, Germany.

Dror Liran (D)

Racah Institute of Physics, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.
The Center for Nanoscience and Nanotechnology, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.

Boaz Lubotzky (B)

Racah Institute of Physics, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.
The Center for Nanoscience and Nanotechnology, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.

Lars Lüder (L)

Institute for Applied Physics and Center LISA+, University of Tuebingen, Auf der Morgenstelle 10, 72076, Tuebingen, Germany.

Monika Fleischer (M)

Institute for Applied Physics and Center LISA+, University of Tuebingen, Auf der Morgenstelle 10, 72076, Tuebingen, Germany.

Ronen Rapaport (R)

Racah Institute of Physics, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.
The Center for Nanoscience and Nanotechnology, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.
The Applied Physics Department, The Hebrew University of Jerusalem, Jerusalem 9190401, Israel.

Classifications MeSH