Quasi-1D exciton channels in strain-engineered 2D materials.


Journal

Science advances
ISSN: 2375-2548
Titre abrégé: Sci Adv
Pays: United States
ID NLM: 101653440

Informations de publication

Date de publication:
29 Oct 2021
Historique:
entrez: 29 10 2021
pubmed: 30 10 2021
medline: 30 10 2021
Statut: ppublish

Résumé

Strain engineering is a powerful tool in designing artificial platforms for high-temperature excitonic quantum devices. Combining strong light-matter interaction with robust and mobile exciton quasiparticles, two-dimensional transition metal dichalcogenides (2D TMDCs) hold great promise in this endeavor. However, realizing complex excitonic architectures based on strain-induced electronic potentials alone has proven to be exceptionally difficult so far. Here, we demonstrate deterministic strain engineering of both single-particle electronic bandstructure and excitonic many-particle interactions. We create quasi-1D transport channels to confine excitons and simultaneously enhance their mobility through locally suppressed exciton-phonon scattering. Using ultrafast, all-optical injection and time-resolved readout, we realize highly directional exciton flow with up to 100% anisotropy both at cryogenic and room temperatures. The demonstrated fundamental modification of the exciton transport properties in a deterministically strained 2D material with effectively tunable dimensionality has broad implications for both basic solid-state science and emerging technologies.

Identifiants

pubmed: 34714670
doi: 10.1126/sciadv.abj3066
pmc: PMC8555901
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

eabj3066

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Auteurs

Florian Dirnberger (F)

Department of Physics, City College of New York, New York, NY 10031, USA.

Jonas D Ziegler (JD)

Department of Physics, University of Regensburg, 93040 Regensburg, Germany.

Paulo E Faria Junior (PE)

Institute for Theoretical Physics, University of Regensburg, 93040 Regensburg, Germany.

Rezlind Bushati (R)

Department of Physics, City College of New York, New York, NY 10031, USA.
Department of Physics, The Graduate Center, City University of New York, New York, NY 10016, USA.

Takashi Taniguchi (T)

International Center for Materials Nanoarchitectonics, National Institute for Materials Science, Tsukuba, Ibaraki 305-004, Japan.

Kenji Watanabe (K)

Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Ibaraki 305-004, Japan.

Jaroslav Fabian (J)

Institute for Theoretical Physics, University of Regensburg, 93040 Regensburg, Germany.

Dominique Bougeard (D)

Department of Physics, University of Regensburg, 93040 Regensburg, Germany.

Alexey Chernikov (A)

Department of Physics, University of Regensburg, 93040 Regensburg, Germany.
Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP) and Würzburg-Dresden Cluster of Excellence ct.qmat, Dresden University of Technology, Dresden 01187, Germany.

Vinod M Menon (VM)

Department of Physics, City College of New York, New York, NY 10031, USA.
Department of Physics, The Graduate Center, City University of New York, New York, NY 10016, USA.

Classifications MeSH