Real-Time Electron Solvation Induced by Bursts of Laser-Accelerated Protons in Liquid Water.


Journal

Physical review letters
ISSN: 1079-7114
Titre abrégé: Phys Rev Lett
Pays: United States
ID NLM: 0401141

Informations de publication

Date de publication:
29 Oct 2021
Historique:
received: 20 05 2021
accepted: 24 09 2021
entrez: 12 11 2021
pubmed: 13 11 2021
medline: 13 11 2021
Statut: ppublish

Résumé

Understanding the mechanisms of proton energy deposition in matter and subsequent damage formation is fundamental to radiation science. Here we exploit the picosecond (10^{-12}  s) resolution of laser-driven accelerators to track ultrafast solvation dynamics for electrons due to proton radiolysis in liquid water (H_{2}O). Comparing these results with modeling that assumes initial conditions similar to those found in photolysis reveals that solvation time due to protons is extended by >20  ps. Supported by magnetohydrodynamic theory this indicates a highly dynamic phase in the immediate aftermath of the proton interaction that is not accounted for in current models.

Identifiants

pubmed: 34767414
doi: 10.1103/PhysRevLett.127.186001
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

186001

Auteurs

A Prasselsperger (A)

Fakultät für Physik, Ludwig-Maximilians-Universität München, 85748 Garching, Germany.
Centre for Plasma Physics, School of Mathematics and Physics, Queens University Belfast, Belfast BT7 1NN, United Kingdom.

M Coughlan (M)

Centre for Plasma Physics, School of Mathematics and Physics, Queens University Belfast, Belfast BT7 1NN, United Kingdom.

N Breslin (N)

Centre for Plasma Physics, School of Mathematics and Physics, Queens University Belfast, Belfast BT7 1NN, United Kingdom.

M Yeung (M)

Centre for Plasma Physics, School of Mathematics and Physics, Queens University Belfast, Belfast BT7 1NN, United Kingdom.

C Arthur (C)

Centre for Plasma Physics, School of Mathematics and Physics, Queens University Belfast, Belfast BT7 1NN, United Kingdom.

H Donnelly (H)

Centre for Plasma Physics, School of Mathematics and Physics, Queens University Belfast, Belfast BT7 1NN, United Kingdom.

S White (S)

Centre for Plasma Physics, School of Mathematics and Physics, Queens University Belfast, Belfast BT7 1NN, United Kingdom.

M Afshari (M)

Centre for Plasma Physics, School of Mathematics and Physics, Queens University Belfast, Belfast BT7 1NN, United Kingdom.

M Speicher (M)

Fakultät für Physik, Ludwig-Maximilians-Universität München, 85748 Garching, Germany.

R Yang (R)

Fakultät für Physik, Ludwig-Maximilians-Universität München, 85748 Garching, Germany.

B Villagomez-Bernabe (B)

The Dalton Cumbria Facility and the School of Chemistry, The University of Manchester, Oxford Rd, Manchester M13 9PL, United Kingdom.

F J Currell (FJ)

The Dalton Cumbria Facility and the School of Chemistry, The University of Manchester, Oxford Rd, Manchester M13 9PL, United Kingdom.

J Schreiber (J)

Fakultät für Physik, Ludwig-Maximilians-Universität München, 85748 Garching, Germany.

B Dromey (B)

Centre for Plasma Physics, School of Mathematics and Physics, Queens University Belfast, Belfast BT7 1NN, United Kingdom.

Classifications MeSH