Real-Time Electron Solvation Induced by Bursts of Laser-Accelerated Protons in Liquid Water.
Journal
Physical review letters
ISSN: 1079-7114
Titre abrégé: Phys Rev Lett
Pays: United States
ID NLM: 0401141
Informations de publication
Date de publication:
29 Oct 2021
29 Oct 2021
Historique:
received:
20
05
2021
accepted:
24
09
2021
entrez:
12
11
2021
pubmed:
13
11
2021
medline:
13
11
2021
Statut:
ppublish
Résumé
Understanding the mechanisms of proton energy deposition in matter and subsequent damage formation is fundamental to radiation science. Here we exploit the picosecond (10^{-12} s) resolution of laser-driven accelerators to track ultrafast solvation dynamics for electrons due to proton radiolysis in liquid water (H_{2}O). Comparing these results with modeling that assumes initial conditions similar to those found in photolysis reveals that solvation time due to protons is extended by >20 ps. Supported by magnetohydrodynamic theory this indicates a highly dynamic phase in the immediate aftermath of the proton interaction that is not accounted for in current models.
Identifiants
pubmed: 34767414
doi: 10.1103/PhysRevLett.127.186001
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM