Cyclopentane peptide nucleic acid: Gold nanoparticle conjugates for the detection of nucleic acids in a microfluidic format.


Journal

Biopolymers
ISSN: 1097-0282
Titre abrégé: Biopolymers
Pays: United States
ID NLM: 0372525

Informations de publication

Date de publication:
Mar 2022
Historique:
revised: 19 10 2021
received: 19 07 2021
accepted: 25 10 2021
pubmed: 24 11 2021
medline: 26 3 2022
entrez: 23 11 2021
Statut: ppublish

Résumé

Routine patient testing for viral infections is critical to identify infected individuals for treatment and to prevent spreading of infections to others. Developing robust and reliable diagnostic tools to detect nucleic acids of viruses at the point-of-care could greatly assist the clinical management of viral infections. The remarkable stability and high binding affinity of peptide nucleic acids (PNAs) to target nucleic acids could make PNA-based biosensors an excellent starting point to develop new nucleic acid detection technologies. We report the application of cyclopentane-modified PNAs to capture target nucleic acids in a microfluidic channel, and the use of bioorthogonal PNAs conjugated to gold nanoparticles as probes to semi-quantitatively signal the presence of a target nucleic acid derived from HIV-1. The basic results presented could be used to develop more advanced devices to detect nucleic acids from viruses such as HIV, SARS-CoV-2, and a wide range of other human diseases.

Identifiants

pubmed: 34812507
doi: 10.1002/bip.23481
pmc: PMC8957522
mid: NIHMS1752587
doi:

Substances chimiques

Cyclopentanes 0
Nucleic Acids 0
Peptide Nucleic Acids 0
Gold 7440-57-5

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e23481

Subventions

Organisme : Office of AIDS Research
Organisme : Intramural NIH HHS
ID : Z01 DK031119
Pays : United States
Organisme : Intramural NIH HHS
ID : ZIA DK031143
Pays : United States
Organisme : Intramural NIH HHS
ID : Z01 DK031143
Pays : United States
Organisme : NIBIB NIH HHS
Pays : United States
Organisme : NIH HHS
Pays : United States
Organisme : NIDDK NIH HHS
Pays : United States

Informations de copyright

© 2021 Wiley Periodicals LLC. This article has been contributed to by US Government employees and their work is in the public domain in the USA.

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Auteurs

Harsha Amarasekara (H)

Synthetic Bioactive Molecules Section, Laboratory of Bioorganic Chemistry (LBC), National Institute of Diabetes and Digestive and Kidney Diseases, National Institutes of Health, Bethesda, Maryland, USA.

Kaylyn M Oshaben (KM)

Synthetic Bioactive Molecules Section, Laboratory of Bioorganic Chemistry (LBC), National Institute of Diabetes and Digestive and Kidney Diseases, National Institutes of Health, Bethesda, Maryland, USA.
Department of Research and Development, Altratech Ltd., Cork, Ireland.

Kendra B Jeans (KB)

Synthetic Bioactive Molecules Section, Laboratory of Bioorganic Chemistry (LBC), National Institute of Diabetes and Digestive and Kidney Diseases, National Institutes of Health, Bethesda, Maryland, USA.

Paniz Rezvan Sangsari (P)

Biomedical Engineering and Physical Science Shared Resource, National Institute of Biomedical Imaging and Bioengineering, National Institutes of Health, Bethesda, Maryland, USA.

Nicole Y Morgan (NY)

Biomedical Engineering and Physical Science Shared Resource, National Institute of Biomedical Imaging and Bioengineering, National Institutes of Health, Bethesda, Maryland, USA.

Brian O'Farrell (B)

Department of Research and Development, Altratech Ltd., Cork, Ireland.

Daniel H Appella (DH)

Synthetic Bioactive Molecules Section, Laboratory of Bioorganic Chemistry (LBC), National Institute of Diabetes and Digestive and Kidney Diseases, National Institutes of Health, Bethesda, Maryland, USA.

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Classifications MeSH