Double-responsive hyaluronic acid-based prodrugs for efficient tumour targeting.


Journal

Materials science & engineering. C, Materials for biological applications
ISSN: 1873-0191
Titre abrégé: Mater Sci Eng C Mater Biol Appl
Pays: Netherlands
ID NLM: 101484109

Informations de publication

Date de publication:
Dec 2021
Historique:
received: 17 06 2021
revised: 30 09 2021
accepted: 01 10 2021
entrez: 3 12 2021
pubmed: 4 12 2021
medline: 15 12 2021
Statut: ppublish

Résumé

Hyaluronic acid (HA)-based prodrugs bearing double-responsive (acid pH or oxidation) boronates of catechol-containing drugs were used to treat xenografted human prostate tumours (LNCaP) in SCID mice. The HA prodrugs accumulated significantly only in tumours (impressively, up to 40% of the injected dose after 24 h) and in liver, with negligible - actually anti-inflammatory - consequences in the latter. A quercetin-HA prodrug significantly slowed down tumour growth, in a dose-dependent fashion and with a much higher efficacy (up to 4 times) than equivalent doses of free quercetin. In short, boronated HA appears to be a very promising platform for targeted chemotherapy.

Identifiants

pubmed: 34857264
pii: S0928-4931(21)00615-9
doi: 10.1016/j.msec.2021.112475
pii:
doi:

Substances chimiques

Micelles 0
Prodrugs 0
Hyaluronic Acid 9004-61-9

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

112475

Informations de copyright

Copyright © 2021 The Authors. Published by Elsevier B.V. All rights reserved.

Auteurs

Vincenzo Quagliariello (V)

Department of Cardio-Thoracic and Respiratory Science, University of Campania "Luigi Vanvitelli", 80138 Napoli, Italy.

Arianna Gennari (A)

Laboratory for Polymers and Biomaterials, Fondazione Istituto Italiano di Tecnologia, 16163 Genova, Italy.

Som Akshay Jain (SA)

Department of Cardio-Thoracic and Respiratory Science, University of Campania "Luigi Vanvitelli", 80138 Napoli, Italy.

Francesco Rosso (F)

Department of Cardio-Thoracic and Respiratory Science, University of Campania "Luigi Vanvitelli", 80138 Napoli, Italy.

Rosario Vincenzo Iaffaioli (RV)

Association for Multidisciplinary Studies in Oncology and Mediterranean Diet, 80138 Napoli, Italy.

Alfonso Barbarisi (A)

Department of Human Sciences, Pegaso Online University, 80132 Napoli, Italy.

Manlio Barbarisi (M)

Department of Medical, Surgical, Neurological, Metabolic and Aging Sciences, University of Campania "Luigi Vanvitelli", 80138 Naples, Italy.

Nicola Tirelli (N)

Laboratory for Polymers and Biomaterials, Fondazione Istituto Italiano di Tecnologia, 16163 Genova, Italy; Division of Pharmacy and Optometry, School of Health Sciences, University of Manchester, Oxford Road, Manchester M13 9PT, United Kingdom. Electronic address: Nicola.tirelli@iit.it.

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Classifications MeSH