The Sensitization of Scintillation in Polymeric Composites Based on Fluorescent Nanocomplexes.
energy transfer
hybrid materials
metal clusters
nanocomposites
nanoscintillators
scintillation
Journal
Nanomaterials (Basel, Switzerland)
ISSN: 2079-4991
Titre abrégé: Nanomaterials (Basel)
Pays: Switzerland
ID NLM: 101610216
Informations de publication
Date de publication:
14 Dec 2021
14 Dec 2021
Historique:
received:
10
11
2021
revised:
05
12
2021
accepted:
09
12
2021
entrez:
24
12
2021
pubmed:
25
12
2021
medline:
25
12
2021
Statut:
epublish
Résumé
The sensitization of scintillation was investigated in crosslinked polymeric composite materials loaded with luminescent gold clusters aggregates acting as sensitizers, and with organic dye rhodamine 6G as the emitting species. The evolution in time of the excited states population in the systems is described by a set of coupled rate equations, in which steady state solution allowed obtainment of an expression of the sensitization efficacy as a function of the characteristic parameters of the employed luminescent systems. The results obtained indicate that the realization of sensitizer/emitter scintillating complexes is the strategy that must be pursued to maximize the sensitization effect in composite materials.
Identifiants
pubmed: 34947738
pii: nano11123387
doi: 10.3390/nano11123387
pmc: PMC8704871
pii:
doi:
Types de publication
Journal Article
Langues
eng
Subventions
Organisme : Italian Ministry of Health (project code RF-2016-02362263, NanoTrack-EXO)
ID : RF-2016-02362263
Organisme : Marie Skłodowska-Curie Actions Widening Fellowships MSCA-WF
ID : grant n° 101003405 - HANSOME
Organisme : Operational Programme Research, Development and Education financed by European Structural and Investment Funds and the Czech Ministry of Education, Youth and Sports
ID : SOLID21 CZ.02.1.01/0.0/0.0/16_019/0000760
Références
Nature. 2020 Nov;587(7835):594-599
pubmed: 33239799
Nanoscale. 2015 Mar 19;7(13):5744-51
pubmed: 25746211
J Am Chem Soc. 2017 Jul 19;139(28):9412-9418
pubmed: 28640637
Adv Mater. 2018 Jul;30(27):e1706956
pubmed: 29736994
Science. 2016 Aug 5;353(6299):571-5
pubmed: 27493181
Nat Nanotechnol. 2020 Jun;15(6):462-468
pubmed: 32424340
Proc Natl Acad Sci U S A. 1978 Dec;75(12):5746-50
pubmed: 16592590
J Mater Chem C Mater. 2013 Mar 14;1(10):1970-1976
pubmed: 26478816
ACS Omega. 2019 May 24;4(5):9169-9180
pubmed: 31460005
Sci Rep. 2017 Aug 4;7(1):7314
pubmed: 28779139