Accurate X-ray Absorption Spectra near L- and M-Edges from Relativistic Four-Component Damped Response Time-Dependent Density Functional Theory.


Journal

Inorganic chemistry
ISSN: 1520-510X
Titre abrégé: Inorg Chem
Pays: United States
ID NLM: 0366543

Informations de publication

Date de publication:
17 Jan 2022
Historique:
pubmed: 28 12 2021
medline: 28 12 2021
entrez: 27 12 2021
Statut: ppublish

Résumé

The simulation of X-ray absorption spectra requires both scalar and spin-orbit (SO) relativistic effects to be taken into account, particularly near L- and M-edges where the SO splitting of core p and d orbitals dominates. Four-component Dirac-Coulomb Hamiltonian-based linear damped response time-dependent density functional theory (4c-DR-TDDFT) calculates spectra directly for a selected frequency region while including the relativistic effects variationally, making the method well suited for X-ray applications. In this work, we show that accurate X-ray absorption spectra near L

Identifiants

pubmed: 34958215
doi: 10.1021/acs.inorgchem.1c02412
pmc: PMC8767545
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

830-846

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Auteurs

Lukas Konecny (L)

Hylleraas Centre for Quantum Molecular Sciences, Department of Chemistry, University of Tromsø - The Arctic University of Norway, 9037 Tromsø, Norway.

Jan Vicha (J)

Centre of Polymer Systems, Tomas Bata University, tř. Tomáše Bati 5678, 760 01 Zlín, Czech Republic.

Stanislav Komorovsky (S)

Institute of Inorganic Chemistry, Slovak Academy of Sciences, Dúbravská cesta 9, SK-84536 Bratislava, Slovakia.

Kenneth Ruud (K)

Hylleraas Centre for Quantum Molecular Sciences, Department of Chemistry, University of Tromsø - The Arctic University of Norway, 9037 Tromsø, Norway.

Michal Repisky (M)

Hylleraas Centre for Quantum Molecular Sciences, Department of Chemistry, University of Tromsø - The Arctic University of Norway, 9037 Tromsø, Norway.

Classifications MeSH