The temperature and flow dependence of nitrate concentration and load estimates based on diffusive gradients in thin films.
Journal
Journal of environmental quality
ISSN: 1537-2537
Titre abrégé: J Environ Qual
Pays: United States
ID NLM: 0330666
Informations de publication
Date de publication:
Mar 2022
Mar 2022
Historique:
received:
10
05
2021
accepted:
20
12
2021
pubmed:
8
1
2022
medline:
24
3
2022
entrez:
7
1
2022
Statut:
ppublish
Résumé
Concentrations determined using diffusive gradients in thin films (DGT) have been used to derive time-averaged loads in streams and rivers. However, DGT provide time-weighted average concentrations that assume the independence of concentration and flow. Additionally, dynamic and coordinated changes in temperature, flow, and concentration are potential sources of bias in concentration and load calculations. We modeled scenarios in which temperature and flow were correlated to varying degrees with concentration and evaluated the consequences for DGT concentration and load calculations. As the correlation between solution flow and concentration moved toward 1 and -1, the load determined by DGT either overestimated or underestimated the actual load by as much as 30%. In DGT-based load estimates, the degree of potential bias should be assessed, and the concentration-flow relation should be characterized. As the correlation of analyte concentration and temperature approached 1 and -1, the deviation of the concentration determined by DGT from the actual concentration increased. In most cases, this bias was < 2%; however, if the changes in concentration and temperature were large (∼10 mg L
Substances chimiques
Nitrates
0
Water Pollutants, Chemical
0
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
250-259Subventions
Organisme : Wellcome Trust
ID : 106835
Pays : United Kingdom
Organisme : Rutherford Discovery Fellowship
ID : RDF-UOW1601
Organisme : Wellcome Trust
ID : 105473
Pays : United Kingdom
Organisme : Wellcome Trust
ID : 106835
Pays : United Kingdom
Organisme : Wellcome Trust
ID : 105473
Pays : United Kingdom
Informations de copyright
© 2022 The Authors. Journal of Environmental Quality © 2022 American Society of Agronomy, Crop Science Society of America, and Soil Science Society of America.
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