Nanoscale-Resolved Surface-to-Bulk Electron Transport in CsPbBr

diffusion electronic structure lead halide perovskites nanoscale charge carrier transport semiconductors ultrafast photoelectron spectroscopy

Journal

Nano letters
ISSN: 1530-6992
Titre abrégé: Nano Lett
Pays: United States
ID NLM: 101088070

Informations de publication

Date de publication:
09 Feb 2022
Historique:
pubmed: 20 1 2022
medline: 20 1 2022
entrez: 19 1 2022
Statut: ppublish

Résumé

Describing the nanoscale charge carrier transport at surfaces and interfaces is fundamental for designing high-performance optoelectronic devices. To achieve this, we employ time- and angle-resolved photoelectron spectroscopy with ultraviolet pump and extreme ultraviolet probe pulses. The resulting high surface sensitivity reveals an ultrafast carrier population decay associated with surface-to-bulk transport, which was tracked with a sub-nanometer spatial resolution normal to the surface, and on a femtosecond time scale, in the case of the inorganic CsPbBr

Identifiants

pubmed: 35044784
doi: 10.1021/acs.nanolett.1c03941
pmc: PMC8832496
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

1067-1074

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Auteurs

Serhii Polishchuk (S)

Laboratoire de Spectroscopie Ultrarapide (LSU) and Lausanne Centre for Ultrafast Science (LACUS), École Polytechnique Fédérale de Lausanne, ISIC, 1015 Lausanne, Switzerland.

Michele Puppin (M)

Laboratoire de Spectroscopie Ultrarapide (LSU) and Lausanne Centre for Ultrafast Science (LACUS), École Polytechnique Fédérale de Lausanne, ISIC, 1015 Lausanne, Switzerland.

Alberto Crepaldi (A)

Institute of Physics and Lausanne Centre for Ultrafast Science (LACUS), École Polytechnique Fédérale de Lausanne, 1015 Lausanne, Switzerland.
Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, Milan 20133, Italy.

Gianmarco Gatti (G)

Institute of Physics and Lausanne Centre for Ultrafast Science (LACUS), École Polytechnique Fédérale de Lausanne, 1015 Lausanne, Switzerland.

Dmitry N Dirin (DN)

Laboratory of Inorganic Chemistry, Department of Chemistry and Applied Biosciences, ETH Zürich, Vladimir-Prelog Weg 1, 8093 Zürich, Switzerland.
Laboratory for Thin Films and Photovoltaics, EMPA-Swiss Federal Laboratories for Materials Science and Technology, Überlandstrasse 129, 8600 Dübendorf, Switzerland.

Olga Nazarenko (O)

Laboratory of Inorganic Chemistry, Department of Chemistry and Applied Biosciences, ETH Zürich, Vladimir-Prelog Weg 1, 8093 Zürich, Switzerland.
Laboratory for Thin Films and Photovoltaics, EMPA-Swiss Federal Laboratories for Materials Science and Technology, Überlandstrasse 129, 8600 Dübendorf, Switzerland.

Nicola Colonna (N)

Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institute, 5232 Villigen-PSI, Switzerland.
National Centre for Computational Design and Discovery of Novel Materials (MARVEL), École Polytechnique Fédérale de Lausanne, 1015 Lausanne, Switzerland.

Nicola Marzari (N)

National Centre for Computational Design and Discovery of Novel Materials (MARVEL), École Polytechnique Fédérale de Lausanne, 1015 Lausanne, Switzerland.

Maksym V Kovalenko (MV)

Laboratory of Inorganic Chemistry, Department of Chemistry and Applied Biosciences, ETH Zürich, Vladimir-Prelog Weg 1, 8093 Zürich, Switzerland.
Laboratory for Thin Films and Photovoltaics, EMPA-Swiss Federal Laboratories for Materials Science and Technology, Überlandstrasse 129, 8600 Dübendorf, Switzerland.

Marco Grioni (M)

Institute of Physics and Lausanne Centre for Ultrafast Science (LACUS), École Polytechnique Fédérale de Lausanne, 1015 Lausanne, Switzerland.

Majed Chergui (M)

Laboratoire de Spectroscopie Ultrarapide (LSU) and Lausanne Centre for Ultrafast Science (LACUS), École Polytechnique Fédérale de Lausanne, ISIC, 1015 Lausanne, Switzerland.

Classifications MeSH