Coloration in Supraparticles Assembled from Polyhedral Metal-Organic Framework Particles.
Emulsion
Metal-Organic Frameworks
Self-Assembly
Structural Color
Supraparticles
Journal
Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543
Informations de publication
Date de publication:
11 Apr 2022
11 Apr 2022
Historique:
received:
22
12
2021
pubmed:
8
2
2022
medline:
8
2
2022
entrez:
7
2
2022
Statut:
ppublish
Résumé
Supraparticles are spherical colloidal crystals prepared by confined self-assembly processes. A particularly appealing property of these microscale structures is the structural color arising from interference of light with their building blocks. Here, we assemble supraparticles with high structural order that exhibit coloration from uniform, polyhedral metal-organic framework (MOF) particles. We analyse the structural coloration as a function of the size of these anisotropic building blocks and their internal structure. We attribute the angle-dependent coloration of the MOF supraparticles to the presence of ordered, onion-like layers at the outermost regions. Surprisingly, even though different shapes of the MOF particles have different propensities to form these onion layers, all supraparticle dispersions show well-visible macroscopic coloration, indicating that local ordering is sufficient to generate interference effects.
Identifiants
pubmed: 35129874
doi: 10.1002/anie.202117455
pmc: PMC9307011
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e202117455Subventions
Organisme : Ministerio de Economía, Industria y Competitividad, Gobierno de España
ID : RTI2018-095622-B-I00
Organisme : Deutsche Forschungsgemeinschaft
ID : 416229255
Informations de copyright
© 2022 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH.
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