Photochemical transformation of hexachlorobenzene (HCB) in solid-water system: Kinetics, mechanism and toxicity evaluation.

Density functional theory Hexachlorobenzene Photodegradation Reaction pathways Reactive oxygen species Silica gel

Journal

Chemosphere
ISSN: 1879-1298
Titre abrégé: Chemosphere
Pays: England
ID NLM: 0320657

Informations de publication

Date de publication:
May 2022
Historique:
received: 07 12 2021
revised: 19 01 2022
accepted: 04 02 2022
pubmed: 14 2 2022
medline: 16 3 2022
entrez: 13 2 2022
Statut: ppublish

Résumé

As one of the first batch of persistent organic pollutants (POPs) included in Stockholm Convention, hexachlorobenzene (HCB) has attracted great attention because of its wide occurrence and great environmental risks. Considering the easy adsorption of HCB on solids and the complexity of natural particles, we systematically investigated the photodegradation of HCB on the surface of silica gel (SG) in aqueous solution in this work to reveal its fate in natural waters. Under mercury lamp irradiation, more than 90% of HCB loaded on SG could be removed after 240 min. Moreover, the effects of solution pH and water constituents were examined, and results showed that the presence of NO

Identifiants

pubmed: 35151701
pii: S0045-6535(22)00400-3
doi: 10.1016/j.chemosphere.2022.133907
pii:
doi:

Substances chimiques

Humic Substances 0
Water 059QF0KO0R
Hexachlorobenzene 4Z87H0LKUY

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

133907

Informations de copyright

Copyright © 2022 Elsevier Ltd. All rights reserved.

Auteurs

Zhengnan Tu (Z)

State Key Laboratory of Pollution Control and Resources Reuse, School of the Environment, Nanjing University, Jiangsu, Nanjing, 210023, PR China.

Yumeng Qi (Y)

State Key Laboratory of Pollution Control and Resources Reuse, School of the Environment, Nanjing University, Jiangsu, Nanjing, 210023, PR China.

Ruijuan Qu (R)

State Key Laboratory of Pollution Control and Resources Reuse, School of the Environment, Nanjing University, Jiangsu, Nanjing, 210023, PR China. Electronic address: quruijuan0404@nju.edu.cn.

Xiaosheng Tang (X)

Jiangsu Yangtze River Delta Environmental Science and Technology Research Institute Co., Ltd., Jiangsu, Changzhou, 213100, PR China.

Zunyao Wang (Z)

State Key Laboratory of Pollution Control and Resources Reuse, School of the Environment, Nanjing University, Jiangsu, Nanjing, 210023, PR China.

Zongli Huo (Z)

Jiangsu Provincial Center for Disease Control and Prevention, No.172 Jiangsu Road, Jiangsu, Nanjing, 210009, PR China.

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Classifications MeSH