Comparative Evaluation of Graphene Nanostructures in GERS Platforms for Pesticide Detection.


Journal

ACS omega
ISSN: 2470-1343
Titre abrégé: ACS Omega
Pays: United States
ID NLM: 101691658

Informations de publication

Date de publication:
22 Feb 2022
Historique:
received: 03 09 2021
accepted: 22 12 2021
entrez: 28 2 2022
pubmed: 1 3 2022
medline: 1 3 2022
Statut: epublish

Résumé

Graphene-enhanced Raman scattering (GERS) produces enhancement of the Raman signal, which is based on chemical rather than electromagnetic mechanism such as in the surface-enhanced Raman scattering. Graphene oxide, amino- and guanidine-functionalized graphene oxide, exfoliated graphene, and commercial graphene nanoplatelets have been used to investigate the GERS response with the change of graphene properties. Different graphene nanostructures have been embedded into organic-inorganic microporous films to build a platform for the fast and sensitive detection of pesticides in water. The graphene nanostructures vary in the number of layers, lateral size, degree of oxidation, and surface functionalization. The GERS performances of the graphene nanostructures cast on silicon substrates and embedded in the nanocomposite films have been comparatively evaluated. After casting a few droplets of the pesticide aqueous solution on the graphene nanostructures, the Raman band enhancements of the analytes have been measured. In the nanocomposite films, the characteristic Raman bands originating from pesticides such as paraoxon, parathion, and glyphosate could be traced at concentrations below 10

Identifiants

pubmed: 35224328
doi: 10.1021/acsomega.1c04863
pmc: PMC8867560
doi:

Types de publication

Journal Article

Langues

eng

Pagination

5670-5678

Informations de copyright

© 2022 The Authors. Published by American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

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Auteurs

Swapneel Thakkar (S)

LMNT, CR-INSTM, Department of Biomedical Sciences, University of Sassari, Viale S. Pietro, 43c, 07100 Sassari SS, Italy.

Lidia De Luca (L)

Department of Chemistry and Pharmacy, University of Sassari, Via Vienna 2, 07100 Sassari, Italy.

Silvia Gaspa (S)

Department of Chemistry and Pharmacy, University of Sassari, Via Vienna 2, 07100 Sassari, Italy.

Alberto Mariani (A)

Department of Chemistry and Pharmacy, University of Sassari, Via Vienna 2, 07100 Sassari, Italy.

Sebastiano Garroni (S)

Department of Chemistry and Pharmacy, University of Sassari, Via Vienna 2, 07100 Sassari, Italy.

Antonio Iacomini (A)

Department of Chemistry and Pharmacy, University of Sassari, Via Vienna 2, 07100 Sassari, Italy.

Luigi Stagi (L)

LMNT, CR-INSTM, Department of Biomedical Sciences, University of Sassari, Viale S. Pietro, 43c, 07100 Sassari SS, Italy.
Department of Chemistry and Pharmacy, University of Sassari, Via Vienna 2, 07100 Sassari, Italy.

Plinio Innocenzi (P)

LMNT, CR-INSTM, Department of Biomedical Sciences, University of Sassari, Viale S. Pietro, 43c, 07100 Sassari SS, Italy.

Luca Malfatti (L)

LMNT, CR-INSTM, Department of Biomedical Sciences, University of Sassari, Viale S. Pietro, 43c, 07100 Sassari SS, Italy.

Classifications MeSH