Attosecond photoionisation time delays reveal the anisotropy of the molecular potential in the recoil frame.
Journal
Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555
Informations de publication
Date de publication:
10 Mar 2022
10 Mar 2022
Historique:
received:
14
10
2021
accepted:
04
02
2022
entrez:
11
3
2022
pubmed:
12
3
2022
medline:
12
3
2022
Statut:
epublish
Résumé
Photoionisation time delays carry structural and dynamical information on the target system, including electronic correlation effects in atoms and molecules and electron transport properties at interfaces. In molecules, the electrostatic potential experienced by an outgoing electron depends on the emission direction, which should thus lead to anisotropic time delays. To isolate this effect, information on the orientation of the molecule at the photoionisation instant is required. Here we show how attosecond time delays reflect the anisotropic molecular potential landscape in CF
Identifiants
pubmed: 35273155
doi: 10.1038/s41467-022-28783-x
pii: 10.1038/s41467-022-28783-x
pmc: PMC8913798
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
1242Subventions
Organisme : EC | Horizon 2020 Framework Programme (EU Framework Programme for Research and Innovation H2020)
ID : 641789
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : INST 39/1079
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : INST 39/1078
Organisme : Bundesministerium für Bildung und Forschung (Federal Ministry of Education and Research)
ID : 05K19VF1
Informations de copyright
© 2022. The Author(s).
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