Efficient Electrochemical Nitrate Reduction to Ammonia with Copper-Supported Rhodium Cluster and Single-Atom Catalysts.
Ammonia Synthesis
Copper Nanowires
Electrochemical Nitrate Reduction
Hydrogen Transfer Mechanism
Single-Atom Catalysts
Journal
Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543
Informations de publication
Date de publication:
07 Jun 2022
07 Jun 2022
Historique:
received:
16
02
2022
pubmed:
18
3
2022
medline:
18
3
2022
entrez:
17
3
2022
Statut:
ppublish
Résumé
The electrochemical nitrate reduction reaction (NITRR) provides a promising solution for restoring the imbalance in the global nitrogen cycle while enabling a sustainable and decentralized route to source ammonia. Here, we demonstrate a novel electrocatalyst for NITRR consisting of Rh clusters and single-atoms dispersed onto Cu nanowires (NWs), which delivers a partial current density of 162 mA cm
Identifiants
pubmed: 35297151
doi: 10.1002/anie.202202556
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e202202556Subventions
Organisme : the Chinese Thousand Talents Program for Young Professionals
Organisme : the startup funding from Nankai University
Organisme : the "111" project
ID : B16027
Organisme : the Spanish Ministry of Science & Innovation for the "Ramon y Cajal" Program
ID : RYC- RYC2018-023888-I
Organisme : the Singapore Ministry of Education AcRF Tier 2
ID : 2016-T2-2-153, 2016-T2-1-131
Organisme : AcRF Tier 1
ID : RG7/18 and RG161/19
Organisme : the Early Postdoc Mobility Fellowship
ID : P2ELP2_199800
Informations de copyright
© 2022 Wiley-VCH GmbH.
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