Picosecond pulse-shaping for strong three-dimensional field-free alignment of generic asymmetric-top molecules.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
17 Mar 2022
Historique:
received: 15 09 2020
accepted: 15 02 2022
entrez: 18 3 2022
pubmed: 19 3 2022
medline: 19 3 2022
Statut: epublish

Résumé

Fixing molecules in space is a crucial step for the imaging of molecular structure and dynamics. Here, we demonstrate three-dimensional (3D) field-free alignment of the prototypical asymmetric top molecule indole using elliptically polarized, shaped, off-resonant laser pulses. A truncated laser pulse is produced using a combination of extreme linear chirping and controlled phase and amplitude shaping using a spatial-light-modulator (SLM) based pulse shaper of a broadband laser pulse. The angular confinement is detected through velocity-map imaging of H

Identifiants

pubmed: 35301292
doi: 10.1038/s41467-022-28951-z
pii: 10.1038/s41467-022-28951-z
pmc: PMC8931173
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

1431

Subventions

Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : KU 1527/3
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : AR 4577/4

Informations de copyright

© 2022. The Author(s).

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Auteurs

Terry Mullins (T)

Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany.

Evangelos T Karamatskos (ET)

Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany.
Department of Physics, Universität Hamburg, Luruper Chaussee 149, 22761, Hamburg, Germany.

Joss Wiese (J)

Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany.
Department of Chemistry, Universität Hamburg, Martin-Luther-King-Platz 6, 20146, Hamburg, Germany.
Center for Ultrafast Imaging, Universität of Hamburg, Luruper Chaussee 149, 22761, Hamburg, Germany.

Jolijn Onvlee (J)

Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany.
Center for Ultrafast Imaging, Universität of Hamburg, Luruper Chaussee 149, 22761, Hamburg, Germany.
Institute for Molecules and Materials, Radboud University, Heijendaalseweg 135, 6525 AJ, Nijmegen, The Netherlands.

Arnaud Rouzée (A)

Max Born Institute, Max-Born-Straße 2a, 12489, Berlin, Germany.

Andrey Yachmenev (A)

Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany.
Center for Ultrafast Imaging, Universität of Hamburg, Luruper Chaussee 149, 22761, Hamburg, Germany.

Sebastian Trippel (S)

Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany.
Center for Ultrafast Imaging, Universität of Hamburg, Luruper Chaussee 149, 22761, Hamburg, Germany.

Jochen Küpper (J)

Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany. jochen.kuepper@cfel.de.
Department of Physics, Universität Hamburg, Luruper Chaussee 149, 22761, Hamburg, Germany. jochen.kuepper@cfel.de.
Department of Chemistry, Universität Hamburg, Martin-Luther-King-Platz 6, 20146, Hamburg, Germany. jochen.kuepper@cfel.de.
Center for Ultrafast Imaging, Universität of Hamburg, Luruper Chaussee 149, 22761, Hamburg, Germany. jochen.kuepper@cfel.de.

Classifications MeSH