Double-Lattice Packing of Pentagonal Gold Bipyramids in Supercrystals with Triclinic Symmetry.
evaporation-induced self-assembly
gold bipyramids
pentagonal packing
supercrystals
triclinic structure
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
May 2022
May 2022
Historique:
revised:
11
03
2022
received:
27
01
2022
pubmed:
25
3
2022
medline:
25
3
2022
entrez:
24
3
2022
Statut:
ppublish
Résumé
Pentagonal packing is a long-standing issue and a rich mathematical topic, brought to the fore by recent progress in nanoparticle design. Gold pentagonal bipyramids combine fivefold symmetry and anisotropy and their section varies along the length. In this work, colloidal supercrystals of pentagonal gold bipyramids are obtained in a compact arrangement that generalizes the optimal packing of regular pentagons in the plane. Multimodal investigations reveal a two-particle unit cell with triclinic symmetry, a lower symmetry than that of the building blocks. Monte Carlo computer simulations show that this lattice achieves the densest possible packing. Going beyond pentagons, further simulations show an odd-even effect of the number of sides on the packing: odd-sided bipyramids are non-centrosymmetric and require the double-lattice arrangement to recover inversion symmetry. The supercrystals display a facet-dependent optical response that is promising for sensing, metamaterials applications, and for fundamental studies of self-assembly processes.
Identifiants
pubmed: 35324025
doi: 10.1002/adma.202200883
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2200883Subventions
Organisme : Investissements d'Avenir grant from Labex PALM
ID : ANR-10-LABX-0039-PALM
Organisme : France-BioImaging
ID : ANR10-INBS-04-01
Organisme : Saclay Plant Science
ID : ANR-11-IDEX-0003-02
Informations de copyright
© 2022 Wiley-VCH GmbH.
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