Exact closure and solution for spatial correlations in single-file diffusion.


Journal

Science advances
ISSN: 2375-2548
Titre abrégé: Sci Adv
Pays: United States
ID NLM: 101653440

Informations de publication

Date de publication:
25 Mar 2022
Historique:
entrez: 25 3 2022
pubmed: 26 3 2022
medline: 26 3 2022
Statut: ppublish

Résumé

In single-file transport particles diffuse in narrow channels while not overtaking each other. it is a fundamental model for the tracer subdiffusion observed in confined systems, such as zeolites or carbon nanotubes. This anomalous behavior originates from strong bath-tracer correlations in one dimension. Despite extensive effort, these remained elusive, because they involve an infinite hierarchy of equations. For the symmetric exclusion process, a paradigmatic model of single-file diffusion, we break the hierarchy to unveil and solve a closed exact equation satisfied by these correlations. Beyond quantifying the correlations, the role of this key equation as a tool for interacting particle systems is further demonstrated by its application to out-of-equilibrium situations, other observables, and other representative single-file systems.

Identifiants

pubmed: 35333581
doi: 10.1126/sciadv.abm5043
pmc: PMC8956262
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

eabm5043

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Auteurs

Aurélien Grabsch (A)

Sorbonne Université, CNRS, Laboratoire de Physique Théorique de la Matière Condensée (LPTMC), 4 Place Jussieu, 75005 Paris, France.

Alexis Poncet (A)

Sorbonne Université, CNRS, Laboratoire de Physique Théorique de la Matière Condensée (LPTMC), 4 Place Jussieu, 75005 Paris, France.
Université Lyon, ENS de Lyon, Université Claude Bernard, CNRS, Laboratoire de Physique, F-69342 Lyon, France.

Pierre Rizkallah (P)

Sorbonne Université, CNRS, Laboratoire de Physico-Chimie des Électrolytes et Nanosystèmes Interfaciaux (PHENIX), 4 Place Jussieu, 75005 Paris, France.

Pierre Illien (P)

Sorbonne Université, CNRS, Laboratoire de Physico-Chimie des Électrolytes et Nanosystèmes Interfaciaux (PHENIX), 4 Place Jussieu, 75005 Paris, France.

Olivier Bénichou (O)

Sorbonne Université, CNRS, Laboratoire de Physique Théorique de la Matière Condensée (LPTMC), 4 Place Jussieu, 75005 Paris, France.

Classifications MeSH