Recycled plastic modified bitumen: Evaluation of VOCs and PAHs from laboratory generated fumes.

Asphalt Bitumen Emissions Fuming Polycyclic aromatic hydrocarbons Recycled plastics Volatile organic compounds

Journal

The Science of the total environment
ISSN: 1879-1026
Titre abrégé: Sci Total Environ
Pays: Netherlands
ID NLM: 0330500

Informations de publication

Date de publication:
01 Aug 2022
Historique:
received: 30 01 2022
revised: 26 03 2022
accepted: 31 03 2022
pubmed: 9 4 2022
medline: 7 6 2022
entrez: 8 4 2022
Statut: ppublish

Résumé

A key aspect when investigating the use of recycled plastics in bitumen relates considerably to the issues relating to occupational, health and safety for humans and the environment from a fuming and emissions perspective. This research investigates laboratory-generated fumes in the forms of volatile organic compounds (VOCs), and polycyclic aromatic hydrocarbons (PAHs) generated from producing polymer modified bitumen using five different types of recycled plastics. A comparative analysis of recycled plastic modified bitumen fumes was conducted based on a series of optimized parameters, including working temperatures (160 °C, 180 °C and 200 °C) and polymer contents (1%, 2%, 4% and 6% by weight of bitumen) against neat bitumen and polymer-modified bitumen. Forty-eight volatile organic compounds (VOCs) and sixteen polycyclic aromatic hydrocarbons (PAHs) were quantified using gas chromatography-mass spectrometry (GC-MS). The results from the comparative analysis revealed that the incorporation of recycled plastics could reduce overall emissions from both VOCs and PAHs perspectives. The reduction in emissions can be attributed to the enhancement in thermal stability of the bitumen blend when recycled plastics are added. The reduction rate is heavily dependent on the type and source of recycled plastics used in the blending process. Furthermore, a specific compound concentration analysis of the top-four weighted compounds emitted reveals that the total concentration of emissions can be deceiving as specific compounds can spike when adding recycled plastics in bitumen despite a reduction trend for the overall concentration.

Identifiants

pubmed: 35395294
pii: S0048-9697(22)02130-1
doi: 10.1016/j.scitotenv.2022.155037
pii:
doi:

Substances chimiques

Gases 0
Hydrocarbons 0
Plastics 0
Polycyclic Aromatic Hydrocarbons 0
Volatile Organic Compounds 0
asphalt 8052-42-4

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

155037

Informations de copyright

Copyright © 2022 Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare the following financial interests/personal relationships which may be considered as potential competing interests: Filippo Giustozzi reports financial support was provided by Austroads Ltd.

Auteurs

Yeong Jia Boom (YJ)

Civil and Infrastructure Engineering, Royal Melbourne Institute of Technology (RMIT) University, 376392 Swanston St, VIC, 3000 Melbourne, Australia.

Marie Enfrin (M)

Civil and Infrastructure Engineering, Royal Melbourne Institute of Technology (RMIT) University, 376392 Swanston St, VIC, 3000 Melbourne, Australia.

Stephen Grist (S)

Civil and Infrastructure Engineering, Royal Melbourne Institute of Technology (RMIT) University, 376392 Swanston St, VIC, 3000 Melbourne, Australia.

Filippo Giustozzi (F)

Civil and Infrastructure Engineering, Royal Melbourne Institute of Technology (RMIT) University, 376392 Swanston St, VIC, 3000 Melbourne, Australia. Electronic address: filippo.giustozzi@rmit.edu.au.

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Classifications MeSH