High-Content Lithium Aluminum Titanium Phosphate-Based Composite Solid Electrolyte with Poly(ionic liquid) Binder.

hardness ionic conductivity lithium aluminum titanium phosphate poly(ionic liquid) solid-state electrolyte

Journal

Polymers
ISSN: 2073-4360
Titre abrégé: Polymers (Basel)
Pays: Switzerland
ID NLM: 101545357

Informations de publication

Date de publication:
22 Mar 2022
Historique:
received: 01 03 2022
revised: 09 03 2022
accepted: 10 03 2022
entrez: 12 4 2022
pubmed: 13 4 2022
medline: 13 4 2022
Statut: epublish

Résumé

Solid electrolytes have been regarded as the most promising electrolyte materials for the next generation of flexible electronic devices due to their excellent safety and machinability. Herein, composite solid electrolytes (CSE) with "polymer in ceramic" are prepared by using lithium aluminum titanium phosphate (LATP) as a matrix and modified poly(ionic liquid) as a binder. The results revealed that adding a poly(ionic liquid)-based binder not only endowed good flexibility for solid electrolytes, but also significantly improved the ionic conductivity of the electrolytes. When the content of LATP in the CSE was 50 wt.%, the electrolyte obtained the highest ionic conductivity (1.2 × 10

Identifiants

pubmed: 35406148
pii: polym14071274
doi: 10.3390/polym14071274
pmc: PMC9003079
pii:
doi:

Types de publication

Journal Article

Langues

eng

Subventions

Organisme : National Natural Science Foundation of China
ID : 52003307
Organisme : Natural Science Foundation of Guangdong Province
ID : 2018A0303130204
Organisme : Guangdong Science and Technology Special Fund
ID : 2019067
Organisme : Jieyang Science and Technology Plan Project
ID : 2019031

Références

Nature. 2008 Feb 7;451(7179):652-7
pubmed: 18256660
ACS Appl Mater Interfaces. 2018 Jan 31;10(4):4113-4120
pubmed: 29303244
Chem Rev. 2004 Oct;104(10):4303-417
pubmed: 15669157
Acc Chem Res. 2013 May 21;46(5):1226-38
pubmed: 23282038
ACS Appl Mater Interfaces. 2017 Jul 5;9(26):21773-21780
pubmed: 28598143
Angew Chem Int Ed Engl. 2016 Jan 11;55(2):500-13
pubmed: 26783056
Nano Lett. 2015 Apr 8;15(4):2740-5
pubmed: 25782069
ACS Appl Mater Interfaces. 2017 Mar 1;9(8):7050-7058
pubmed: 28128548
Chem Soc Rev. 2011 May;40(5):2525-40
pubmed: 21253642
Polymers (Basel). 2017 Nov 15;9(11):
pubmed: 30965921
Nature. 2001 Nov 15;414(6861):359-67
pubmed: 11713543

Auteurs

Fujie Yang (F)

GD HPPC Lab, College Chemistry and Chemical Engineering, Zhongkai University of Agriculture and Engineering, Guangzhou 510275, China.

Qingfeng Liu (Q)

GD HPPC Lab, College Chemistry and Chemical Engineering, Zhongkai University of Agriculture and Engineering, Guangzhou 510275, China.

Wenfei Xie (W)

GD HPPC Lab, College Chemistry and Chemical Engineering, Zhongkai University of Agriculture and Engineering, Guangzhou 510275, China.

Pu Xie (P)

School of Chemistry, Sun Yat-Sen University, Guangzhou 510275, China.

Jingqi Shang (J)

GD HPPC Lab, College Chemistry and Chemical Engineering, Zhongkai University of Agriculture and Engineering, Guangzhou 510275, China.

Xugang Shu (X)

GD HPPC Lab, College Chemistry and Chemical Engineering, Zhongkai University of Agriculture and Engineering, Guangzhou 510275, China.

Classifications MeSH