CDP-ribitol prodrug treatment ameliorates ISPD-deficient muscular dystrophy mouse model.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
14 04 2022
Historique:
received: 16 02 2021
accepted: 17 03 2022
entrez: 15 4 2022
pubmed: 16 4 2022
medline: 19 4 2022
Statut: epublish

Résumé

Ribitol-phosphate modification is crucial for the functional maturation of α-dystroglycan. Its dysfunction is associated with muscular dystrophy, cardiomyopathy, and central nervous system abnormalities; however, no effective treatments are currently available for diseases caused by ribitol-phosphate defects. In this study, we demonstrate that prodrug treatments can ameliorate muscular dystrophy caused by defects in isoprenoid synthase domain containing (ISPD), which encodes an enzyme that synthesizes CDP-ribitol, a donor substrate for ribitol-phosphate modification. We generated skeletal muscle-selective Ispd conditional knockout mice, leading to a pathogenic reduction in CDP-ribitol levels, abnormal glycosylation of α-dystroglycan, and severe muscular dystrophy. Adeno-associated virus-mediated gene replacement experiments suggested that the recovery of CDP-ribitol levels rescues the ISPD-deficient pathology. As a prodrug treatment strategy, we developed a series of membrane-permeable CDP-ribitol derivatives, among which tetraacetylated CDP-ribitol ameliorated the dystrophic pathology. In addition, the prodrug successfully rescued abnormal α-dystroglycan glycosylation in patient fibroblasts. Consequently, our findings provide proof-of-concept for supplementation therapy with CDP-ribitol and could accelerate the development of therapeutic agents for muscular dystrophy and other diseases caused by glycosylation defects.

Identifiants

pubmed: 35422047
doi: 10.1038/s41467-022-29473-4
pii: 10.1038/s41467-022-29473-4
pmc: PMC9010444
doi:

Substances chimiques

Dystroglycans 146888-27-9
Phosphates 0
Prodrugs 0
Ribitol 488-81-3

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

1847

Informations de copyright

© 2022. The Author(s).

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Auteurs

Hideki Tokuoka (H)

Division of Molecular Brain Science, Kobe University Graduate School of Medicine, Kobe, Hyogo, 650-0017, Japan.
Division of Neurology, Kobe University Graduate School of Medicine, Kobe, Hyogo, 650-0017, Japan.

Rieko Imae (R)

Molecular Glycobiology, Research Team for Mechanism of Aging, Tokyo Metropolitan Geriatric Hospital and Institute of Gerontology, Itabashi-ku, Tokyo, 173-0015, Japan.

Hitomi Nakashima (H)

Division of Molecular Brain Science, Kobe University Graduate School of Medicine, Kobe, Hyogo, 650-0017, Japan.

Hiroshi Manya (H)

Molecular Glycobiology, Research Team for Mechanism of Aging, Tokyo Metropolitan Geriatric Hospital and Institute of Gerontology, Itabashi-ku, Tokyo, 173-0015, Japan.

Chiaki Masuda (C)

Department of Biochemistry and Molecular Biology, Nippon Medical School, Bunkyo-ku, Tokyo, 113-8602, Japan.

Shunsuke Hoshino (S)

Molecular Glycobiology, Research Team for Mechanism of Aging, Tokyo Metropolitan Geriatric Hospital and Institute of Gerontology, Itabashi-ku, Tokyo, 173-0015, Japan.

Kazuhiro Kobayashi (K)

Division of Molecular Brain Science, Kobe University Graduate School of Medicine, Kobe, Hyogo, 650-0017, Japan.

Dirk J Lefeber (DJ)

Department of Neurology, Donders Institute for Brain, Cognition and Behavior, Radboud University Medical Center, Nijmegen, the Netherlands; Translational Metabolic Laboratory, Department of Laboratory Medicine, Radboud Institute for Molecular Life Sciences, Radboud University Medical Center, 6525 GA, Nijmegen, The Netherlands.

Riki Matsumoto (R)

Division of Neurology, Kobe University Graduate School of Medicine, Kobe, Hyogo, 650-0017, Japan.

Takashi Okada (T)

Division of Molecular and Medical Genetics, Center for Gene and Cell Therapy, The Institute of Medical Science, The University of Tokyo, Minato-ku, Tokyo, 108-8639, Japan.

Tamao Endo (T)

Molecular Glycobiology, Research Team for Mechanism of Aging, Tokyo Metropolitan Geriatric Hospital and Institute of Gerontology, Itabashi-ku, Tokyo, 173-0015, Japan.

Motoi Kanagawa (M)

Division of Molecular Brain Science, Kobe University Graduate School of Medicine, Kobe, Hyogo, 650-0017, Japan. kanagawa.motoi.fa@ehime-u.ac.jp.
Department of Cell Biology and Molecular Medicine, Ehime University Graduate School of Medicine, Toon, Ehime, 791-0295, Japan. kanagawa.motoi.fa@ehime-u.ac.jp.

Tatsushi Toda (T)

Department of Neurology, Graduate School of Medicine, The University of Tokyo, Bunkyo-ku, Tokyo, 113-8655, Japan. toda@m.u-tokyo.ac.jp.

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