Strong Coupling of Carbon Quantum Dots in Liquid Crystals.


Journal

The journal of physical chemistry letters
ISSN: 1948-7185
Titre abrégé: J Phys Chem Lett
Pays: United States
ID NLM: 101526034

Informations de publication

Date de publication:
28 Apr 2022
Historique:
pubmed: 16 4 2022
medline: 16 4 2022
entrez: 15 4 2022
Statut: ppublish

Résumé

Carbon quantum dots (CDs) have recently received a tremendous amount of interest owing to their attractive optical properties. However, CDs have broad absorption and emission spectra limiting their application ranges. We herein, for the first time, show synthesis of water-soluble red emissive CDs with a very narrow line width (∼75 meV) spectral absorbance and hence demonstrate strong coupling of CDs and plasmon polaritons in liquid crystalline mesophases. The excited state dynamics of CDs has been studied by ultrafast transient absorption spectroscopy, and CDs display very stable and strong photoluminescence emission with a quantum yield of 35.4% and a lifetime of ∼2 ns. More importantly, we compare

Identifiants

pubmed: 35426302
doi: 10.1021/acs.jpclett.1c03937
pmc: PMC9059182
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

3562-3570

Références

Nat Commun. 2018 Jun 8;9(1):2249
pubmed: 29884873
J Am Chem Soc. 2007 Jan 31;129(4):744-5
pubmed: 17243794
J Phys Chem Lett. 2016 Nov 17;7(22):4648-4654
pubmed: 27804299
Nano Lett. 2008 Dec;8(12):4248-51
pubmed: 19367881
Adv Mater. 2016 Jan 13;28(2):312-8
pubmed: 26568431
Angew Chem Int Ed Engl. 2015 Apr 27;54(18):5360-3
pubmed: 25832292
J Am Chem Soc. 2006 Jun 21;128(24):7756-7
pubmed: 16771487
Nat Commun. 2021 Feb 26;12(1):1310
pubmed: 33637699
Phys Rev Lett. 2015 Apr 17;114(15):157401
pubmed: 25933338
Nano Lett. 2016 Oct 12;16(10):6504-6510
pubmed: 27661764
J Am Chem Soc. 2004 Oct 13;126(40):12736-7
pubmed: 15469243
Nano Lett. 2011 Aug 10;11(8):3184-9
pubmed: 21696177
Adv Mater. 2020 Apr;32(17):e1906641
pubmed: 32191372
J Phys Chem Lett. 2018 Apr 5;9(7):1676-1681
pubmed: 29547298
Angew Chem Int Ed Engl. 2013 Jul 22;52(30):7800-4
pubmed: 23761198
Sci Adv. 2018 Mar 02;4(3):eaar4906
pubmed: 29511739
Langmuir. 2015 Sep 22;31(37):10265-71
pubmed: 26332603
Nano Lett. 2018 Mar 14;18(3):1777-1785
pubmed: 29369640
Nanoscale. 2017 Feb 2;9(5):1909-1915
pubmed: 28094404

Auteurs

Sema Sarisozen (S)

Department of Chemistry, Izmir Institute of Technology, Izmir 35430, Turkey.

Nahit Polat (N)

Department of Photonics, Izmir Institute of Technology, Izmir 35430, Turkey.

Fadime Mert Balci (F)

Department of Chemistry, Izmir Institute of Technology, Izmir 35430, Turkey.

C Meric Guvenc (CM)

Department of Materials Science and Engineering, Izmir Institute of Technology, Izmir 35430, Turkey.

Coskun Kocabas (C)

Department of Materials, University of Manchester, Manchester M13 9PL, U.K.
National Graphene Institute (NGI), University of Manchester, Manchester M13 9PL, U.K.
Henry Royce Institute for Advanced Materials, University of Manchester, Manchester M13 9PL, U.K.

Halime Gul Yaglioglu (HG)

Department of Engineering Physics, Ankara University, Ankara 06100, Turkey.

Sinan Balci (S)

Department of Photonics, Izmir Institute of Technology, Izmir 35430, Turkey.

Classifications MeSH