Q-dependent collective relaxation dynamics of glass-forming liquid Ca


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
19 Apr 2022
Historique:
received: 21 09 2021
accepted: 29 03 2022
entrez: 20 4 2022
pubmed: 21 4 2022
medline: 21 4 2022
Statut: epublish

Résumé

The relaxation behavior of glass formers exhibits spatial heterogeneity and dramatically changes upon cooling towards the glass transition. However, the underlying mechanisms of the dynamics at different microscopic length scales are not fully understood. Employing the recently developed wide-angle neutron spin-echo spectroscopy technique, we measured the Q-dependent coherent intermediate scattering function of a prototypical ionic glass former Ca

Identifiants

pubmed: 35440658
doi: 10.1038/s41467-022-29778-4
pii: 10.1038/s41467-022-29778-4
pmc: PMC9018732
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

2092

Subventions

Organisme : U.S. Department of Energy (DOE)
ID : DE-SC0014084

Informations de copyright

© 2022. The Author(s).

Références

Phys Rev Lett. 2017 Apr 7;118(14):147801
pubmed: 28430517
Nat Commun. 2021 Mar 25;12(1):1867
pubmed: 33767148
J Phys Chem Lett. 2017 Oct 5;8(19):4679-4684
pubmed: 28892394
Phys Rev Lett. 2015 Oct 2;115(14):148302
pubmed: 26551826
Phys Rev Lett. 2012 Sep 14;109(11):115705
pubmed: 23005649
Proc Natl Acad Sci U S A. 2020 Sep 8;117(36):21896-21905
pubmed: 32843347
Nature. 2001 Mar 8;410(6825):259-67
pubmed: 11258381
Phys Rev Lett. 1996 Mar 11;76(11):1872-1875
pubmed: 10060542
Phys Rev E Stat Nonlin Soft Matter Phys. 2001 Oct;64(4 Pt 1):041503
pubmed: 11690029
Phys Rev Lett. 2002 Dec 9;89(24):245701
pubmed: 12484957
J Phys Chem B. 2013 Mar 7;117(9):2773-81
pubmed: 23391265
Phys Rev Lett. 1992 Sep 7;69(10):1620
pubmed: 10046268
Phys Rev Lett. 1987 Feb 9;58(6):571-574
pubmed: 10034975
Phys Rev Lett. 2020 Jul 31;125(5):055701
pubmed: 32794848
Phys Rev B Condens Matter. 1996 Sep 1;54(9):6292-6300
pubmed: 9986645
J Res Natl Inst Stand Technol. 2009 Dec 01;114(6):341-58
pubmed: 27504233
Science. 2016 Jun 10;352(6291):1308-11
pubmed: 27284191
Phys Rev Lett. 2001 Jun 11;86(24):5526-9
pubmed: 11415292
Phys Rev B Condens Matter. 1992 May 1;45(18):10301-10305
pubmed: 10000933
J Chem Phys. 2011 Aug 7;135(5):054508
pubmed: 21823713
Phys Rev A. 1992 Jan 15;45(2):898-912
pubmed: 9907056
Phys Rev Lett. 2008 Jul 18;101(3):037801
pubmed: 18764296
Phys Chem Chem Phys. 2021 Mar 28;23(12):7220-7232
pubmed: 33876082
J Phys Chem Lett. 2021 Jan 14;12(1):392-398
pubmed: 33356292
Phys Rev Lett. 1992 Jan 6;68(1):71-74
pubmed: 10045115
Phys Rev Lett. 2006 May 12;96(18):185701
pubmed: 16712373
J Chem Phys. 2014 Apr 14;140(14):144906
pubmed: 24735317
J Phys Chem B. 2017 Dec 14;121(49):11210-11218
pubmed: 29166015
Phys Rev Lett. 2000 Apr 17;84(16):3630-3
pubmed: 11019163
Annu Rev Phys Chem. 2000;51:99-128
pubmed: 11031277
Phys Rev Lett. 1985 Jan 14;54(2):118-121
pubmed: 10031259
Proc Natl Acad Sci U S A. 2021 Mar 30;118(13):
pubmed: 33753508
Phys Rev Lett. 1988 Nov 21;61(21):2465-2468
pubmed: 10039125
Science. 2000 Jan 28;287(5453):627-31
pubmed: 10649991
Science. 2005 Dec 16;310(5755):1797-800
pubmed: 16357256

Auteurs

Peng Luo (P)

Beckman Institute for Advanced Science and Technology, University of Illinois at Urbana-Champaign, Urbana, IL, 61801, USA.

Yanqin Zhai (Y)

Beckman Institute for Advanced Science and Technology, University of Illinois at Urbana-Champaign, Urbana, IL, 61801, USA.
Department of Nuclear, Plasma, and Radiological Engineering, University of Illinois at Urbana-Champaign, Urbana, IL, 61801, USA.

Peter Falus (P)

Institut Laue-Langevin (ILL), 38042, Grenoble, France.

Victoria García Sakai (V)

ISIS Neutron and Muon Facility, Rutherford Appleton Laboratory, Science & Technology Facilities Council, Didcot, OX11 0QX, UK.

Monika Hartl (M)

European Spallation Source, SE-221 00, Lund, Sweden.

Maiko Kofu (M)

J-PARC Center, Japan Atomic Energy Agency, Tokai, Ibaraki, 319-1195, Japan.

Kenji Nakajima (K)

J-PARC Center, Japan Atomic Energy Agency, Tokai, Ibaraki, 319-1195, Japan.

Antonio Faraone (A)

NIST Center for Neutron Research, National Institute of Standards and Technology, 100 Bureau Drive, Gaithersburg, MD, 20899-1070, USA. antonio.faraone@nist.gov.

Y Z (Y)

Beckman Institute for Advanced Science and Technology, University of Illinois at Urbana-Champaign, Urbana, IL, 61801, USA. zhyang@illinois.edu.
Department of Nuclear, Plasma, and Radiological Engineering, University of Illinois at Urbana-Champaign, Urbana, IL, 61801, USA. zhyang@illinois.edu.
Department of Electrical and Computer Engineering, University of Illinois at Urbana-Champaign, Urbana, IL, 61801, USA. zhyang@illinois.edu.

Classifications MeSH