Dynamics of particle network in composite battery cathodes.


Journal

Science (New York, N.Y.)
ISSN: 1095-9203
Titre abrégé: Science
Pays: United States
ID NLM: 0404511

Informations de publication

Date de publication:
29 04 2022
Historique:
entrez: 28 4 2022
pubmed: 29 4 2022
medline: 3 5 2022
Statut: ppublish

Résumé

Improving composite battery electrodes requires a delicate control of active materials and electrode formulation. The electrochemically active particles fulfill their role as energy exchange reservoirs through interacting with the surrounding conductive network. We formulate a network evolution model to interpret the regulation and equilibration between electrochemical activity and mechanical damage of these particles. Through statistical analysis of thousands of particles using x-ray phase contrast holotomography in a LiNi

Identifiants

pubmed: 35482882
doi: 10.1126/science.abm8962
doi:

Types de publication

Journal Article Research Support, Non-U.S. Gov't Research Support, U.S. Gov't, Non-P.H.S.

Langues

eng

Sous-ensembles de citation

IM

Pagination

517-521

Auteurs

Jizhou Li (J)

Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

Nikhil Sharma (N)

School of Mechanical Engineering, Purdue University, West Lafayette, IN 47906, USA.

Zhisen Jiang (Z)

Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

Yang Yang (Y)

European Synchrotron Radiation Facility, Grenoble 38000, France.

Federico Monaco (F)

European Synchrotron Radiation Facility, Grenoble 38000, France.

Zhengrui Xu (Z)

Department of Chemistry, Virginia Tech, Blacksburg, VA 24061, USA.

Dong Hou (D)

Department of Chemistry, Virginia Tech, Blacksburg, VA 24061, USA.

Daniel Ratner (D)

Machine Learning Initiative, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

Piero Pianetta (P)

Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

Peter Cloetens (P)

European Synchrotron Radiation Facility, Grenoble 38000, France.

Feng Lin (F)

Department of Chemistry, Virginia Tech, Blacksburg, VA 24061, USA.

Kejie Zhao (K)

School of Mechanical Engineering, Purdue University, West Lafayette, IN 47906, USA.

Yijin Liu (Y)

Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

Classifications MeSH