A cost-effective alkaline polysulfide-air redox flow battery enabled by a dual-membrane cell architecture.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
02 May 2022
Historique:
received: 06 08 2021
accepted: 14 04 2022
entrez: 2 5 2022
pubmed: 3 5 2022
medline: 3 5 2022
Statut: epublish

Résumé

With the rapid development of renewable energy harvesting technologies, there is a significant demand for long-duration energy storage technologies that can be deployed at grid scale. In this regard, polysulfide-air redox flow batteries demonstrated great potential. However, the crossover of polysulfide is one significant challenge. Here, we report a stable and cost-effective alkaline-based hybrid polysulfide-air redox flow battery where a dual-membrane-structured flow cell design mitigates the sulfur crossover issue. Moreover, combining manganese/carbon catalysed air electrodes with sulfidised Ni foam polysulfide electrodes, the redox flow battery achieves a maximum power density of 5.8 mW cm

Identifiants

pubmed: 35501344
doi: 10.1038/s41467-022-30044-w
pii: 10.1038/s41467-022-30044-w
pmc: PMC9061742
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

2388

Subventions

Organisme : RCUK | Engineering and Physical Sciences Research Council (EPSRC)
ID : EP/K002252/1
Organisme : EC | EU Framework Programme for Research and Innovation H2020 | H2020 Priority Excellent Science | H2020 European Research Council (H2020 Excellent Science - European Research Council)
ID : ERC-StG-PE8-NanoMMES

Informations de copyright

© 2022. The Author(s).

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Auteurs

Yuhua Xia (Y)

Department of Earth Science and Engineering, Imperial College London, London, SW7 2AZ, UK.

Mengzheng Ouyang (M)

Department of Earth Science and Engineering, Imperial College London, London, SW7 2AZ, UK. m.ouyang15@imperial.ac.uk.

Vladimir Yufit (V)

Department of Earth Science and Engineering, Imperial College London, London, SW7 2AZ, UK.
Addionics Ltd., Imperial White City Incubator, 80 Wood Lane, London, W12 0BZ, UK.

Rui Tan (R)

Department of Chemical Engineering, Imperial College London, London, SW7 2AZ, UK.

Anna Regoutz (A)

Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, UK.

Anqi Wang (A)

Department of Chemical Engineering, Imperial College London, London, SW7 2AZ, UK.

Wenjie Mao (W)

Department of Chemical Engineering, Imperial College London, London, SW7 2AZ, UK.

Barun Chakrabarti (B)

Department of Earth Science and Engineering, Imperial College London, London, SW7 2AZ, UK.
WMG, Warwick Electrochemical Engineering Group, Energy Innovation Centre, University of Warwick, Coventry, CV4 7AL, UK.

Ashkan Kavei (A)

Department of Earth Science and Engineering, Imperial College London, London, SW7 2AZ, UK.
RFC Power Ltd., Imperial White City Incubator, 80 Wood Lane, London, W12 0BZ, UK.

Qilei Song (Q)

Department of Chemical Engineering, Imperial College London, London, SW7 2AZ, UK.

Anthony R Kucernak (AR)

RFC Power Ltd., Imperial White City Incubator, 80 Wood Lane, London, W12 0BZ, UK.
Department of Chemistry, Imperial College London, London, SW7 2AZ, UK.

Nigel P Brandon (NP)

Department of Earth Science and Engineering, Imperial College London, London, SW7 2AZ, UK.
RFC Power Ltd., Imperial White City Incubator, 80 Wood Lane, London, W12 0BZ, UK.

Classifications MeSH