Hybrid catalysts based on N-heterocyclic carbene anchored on hierarchical zeolites.


Journal

RSC advances
ISSN: 2046-2069
Titre abrégé: RSC Adv
Pays: England
ID NLM: 101581657

Informations de publication

Date de publication:
31 Oct 2019
Historique:
received: 17 09 2019
accepted: 18 10 2019
entrez: 9 5 2022
pubmed: 31 10 2019
medline: 31 10 2019
Statut: epublish

Résumé

Hybrid materials have been synthesized by anchoring a N-heterocyclic carbene (NHC) precursor on different inorganic zeolitic supports with hierarchical porosity, in particular hierarchical HZSM-5 and SAPO-5. Hierarchical porous inorganic supports have been obtained both by top-down and bottom-up approaches and the role of hierarchical porosity has been evaluated. A detailed physico-chemical characterization has been performed on the organic-inorganic hybrids using a multi-technique approach (XRD, volumetric and thermogravimetric analysis, ssNMR and FTIR) in order to establish a structure-property relationship. The hybrids were tested in the benzoin condensation reaction of furfural, a base catalyzed reaction.

Identifiants

pubmed: 35528109
doi: 10.1039/c9ra07516j
pii: c9ra07516j
pmc: PMC9074450
doi:

Types de publication

Journal Article

Langues

eng

Pagination

35336-35344

Informations de copyright

This journal is © The Royal Society of Chemistry.

Déclaration de conflit d'intérêts

There are no conflicts to declare.

Références

Chem Soc Rev. 2017 Jan 23;46(2):481-558
pubmed: 27906387
Chem Soc Rev. 2013 May 7;42(9):4004-35
pubmed: 23138888
Chem Soc Rev. 2018 Jul 30;47(15):5684-5739
pubmed: 30014075
Langmuir. 2004 Dec 7;20(25):10962-9
pubmed: 15568847
Solid State Nucl Magn Reson. 2011 May-Jun;39(3-4):116-41
pubmed: 21592743
Chem Rev. 2011 Apr 13;111(4):2705-33
pubmed: 21235210
Chem Rev. 2002 Oct;102(10):3589-613
pubmed: 12371895
Chem Soc Rev. 2016 Jun 13;45(12):3313-30
pubmed: 26983374
Nature. 2014 Jun 26;510(7506):485-96
pubmed: 24965649
Chem Soc Rev. 2013 May 7;42(9):4083-97
pubmed: 23288312
Angew Chem Int Ed Engl. 2015 Jan 26;54(5):1591-4
pubmed: 25376507
Angew Chem Int Ed Engl. 2002 May 17;41(10):1743-5
pubmed: 19750702
Chem Rev. 2017 Feb 8;117(3):1970-2058
pubmed: 28085269
Chem Rev. 2007 Dec;107(12):5606-55
pubmed: 17956132
Chemistry. 2017 Jul 21;23(41):9952-9961
pubmed: 28574168
Angew Chem Int Ed Engl. 2006 May 12;45(20):3216-51
pubmed: 16676373

Auteurs

Enrica Gianotti (E)

Department of Science and Technological Innovation, Università del Piemonte Orientale V. T. Michel 11 I-15121 Alessandria Italy enrica.gianotti@uniupo.it.

Ivana Miletto (I)

Department of Science and Technological Innovation, Università del Piemonte Orientale V. T. Michel 11 I-15121 Alessandria Italy enrica.gianotti@uniupo.it.

Chiara Ivaldi (C)

Department of Science and Technological Innovation, Università del Piemonte Orientale V. T. Michel 11 I-15121 Alessandria Italy enrica.gianotti@uniupo.it.

Geo Paul (G)

Department of Science and Technological Innovation, Università del Piemonte Orientale V. T. Michel 11 I-15121 Alessandria Italy enrica.gianotti@uniupo.it.

Leonardo Marchese (L)

Department of Science and Technological Innovation, Università del Piemonte Orientale V. T. Michel 11 I-15121 Alessandria Italy enrica.gianotti@uniupo.it.

Marta Meazza (M)

School of Chemistry, University of Southampton University Road Southampton SO17 1BJ UK.

Ramon Rios (R)

School of Chemistry, University of Southampton University Road Southampton SO17 1BJ UK.

Robert Raja (R)

School of Chemistry, University of Southampton University Road Southampton SO17 1BJ UK.

Classifications MeSH