Theory-guided experimental design in battery materials research.
Journal
Science advances
ISSN: 2375-2548
Titre abrégé: Sci Adv
Pays: United States
ID NLM: 101653440
Informations de publication
Date de publication:
13 May 2022
13 May 2022
Historique:
entrez:
11
5
2022
pubmed:
12
5
2022
medline:
12
5
2022
Statut:
ppublish
Résumé
A reliable energy storage ecosystem is imperative for a renewable energy future, and continued research is needed to develop promising rechargeable battery chemistries. To this end, better theoretical and experimental understanding of electrochemical mechanisms and structure-property relationships will allow us to accelerate the development of safer batteries with higher energy densities and longer lifetimes. This Review discusses the interplay between theory and experiment in battery materials research, enabling us to not only uncover hitherto unknown mechanisms but also rationally design more promising electrode and electrolyte materials. We examine specific case studies of theory-guided experimental design in lithium-ion, lithium-metal, sodium-metal, and all-solid-state batteries. We also offer insights into how this framework can be extended to multivalent batteries. To close the loop, we outline recent efforts in coupling machine learning with high-throughput computations and experiments. Last, recommendations for effective collaboration between theorists and experimentalists are provided.
Identifiants
pubmed: 35544561
doi: 10.1126/sciadv.abm2422
pmc: PMC9094674
doi:
Types de publication
Journal Article
Review
Langues
eng
Sous-ensembles de citation
IM
Pagination
eabm2422Références
Top Curr Chem (Cham). 2018 Apr 26;376(3):19
pubmed: 29700688
Science. 2008 Aug 8;321(5890):792-4
pubmed: 18687952
Nat Commun. 2016 Jun 09;7:11722
pubmed: 27277345
ACS Appl Mater Interfaces. 2016 Oct 12;8(40):26842-26850
pubmed: 27642769
Phys Rev Lett. 2017 Aug 4;119(5):056003
pubmed: 28949705
Chem Rev. 2017 Mar 8;117(5):4287-4341
pubmed: 28269988
Nature. 2018 Aug;560(7718):345-349
pubmed: 30111789
Nat Clim Chang. 2020;10(10):971
pubmed: 32845944
Faraday Discuss. 2017 Jul 1;199:423-463
pubmed: 28573280
Nature. 2020 Feb;578(7795):397-402
pubmed: 32076218
Chem Commun (Camb). 2014 Jan 7;50(2):243-5
pubmed: 24225903
Anal Chem. 2017 Aug 1;89(15):8122-8128
pubmed: 28669177
Mater Horiz. 2021 Mar 1;8(3):830-853
pubmed: 34821317
Chem Rev. 2014 Dec 10;114(23):11414-43
pubmed: 25354149
Nat Mater. 2015 Oct;14(10):1026-31
pubmed: 26280225
Chem Rev. 2022 Jun 22;122(12):10899-10969
pubmed: 34529918
Nature. 2001 Nov 15;414(6861):359-67
pubmed: 11713543
Nat Chem. 2016 Jul;8(7):684-91
pubmed: 27325095
J Am Chem Soc. 2015 Apr 15;137(14):4804-14
pubmed: 25811894
Phys Chem Chem Phys. 2015 Jun 7;17(21):13949-63
pubmed: 25947073
Chem Rev. 2014 Dec 10;114(23):11683-720
pubmed: 25343313
Acc Chem Res. 2017 Apr 18;50(4):1022-1031
pubmed: 28300397
Phys Chem Chem Phys. 2014 Oct 28;16(40):22073-82
pubmed: 25209334
Nat Mater. 2017 Nov;16(11):1142-1148
pubmed: 28920941
Phys Rev Lett. 2011 Sep 9;107(11):118301
pubmed: 22026706
ACS Cent Sci. 2015 Nov 25;1(8):449-55
pubmed: 27163006
Chem Rev. 2019 Apr 10;119(7):4569-4627
pubmed: 30859816
Chem Soc Rev. 2019 Apr 1;48(7):1865-1873
pubmed: 30869084
ACS Comb Sci. 2016 Jun 13;18(6):343-8
pubmed: 27124559
Nat Commun. 2018 Sep 24;9(1):3870
pubmed: 30250202
Chem Sci. 2020 Jul 30;11(32):8517-8532
pubmed: 34123112
Nat Commun. 2013;4:1331
pubmed: 23299881
Nat Commun. 2018 Jan 31;9(1):464
pubmed: 29386598
Nat Commun. 2019 Nov 20;10(1):5260
pubmed: 31748523
Chem Rev. 2020 Jul 22;120(14):6977-7019
pubmed: 32022553
Chem Rev. 2020 Jul 22;120(14):6558-6625
pubmed: 32090540
ACS Appl Mater Interfaces. 2019 May 22;11(20):18494-18503
pubmed: 31034195
Sci Adv. 2020 Aug 07;6(32):eabb1342
pubmed: 32821832
Sci Rep. 2016 Jun 16;6:28054
pubmed: 27307136
Science. 2019 Nov 22;366(6468):
pubmed: 31753970
Phys Chem Chem Phys. 2015 Nov 21;17(43):28441-50
pubmed: 26076998
Nature. 2000 Oct 12;407(6805):724-7
pubmed: 11048714
Sci Data. 2020 Sep 8;7(1):300
pubmed: 32901044
PLoS One. 2015 Jul 10;10(7):e0130140
pubmed: 26161953
Chem Soc Rev. 2016 Oct 21;45(20):5605-5634
pubmed: 27460222
Nat Nanotechnol. 2017 Mar 7;12(3):194-206
pubmed: 28265117
Nat Mater. 2020 Oct;19(10):1096-1101
pubmed: 32367080
Adv Mater. 2019 Feb;31(5):e1802822
pubmed: 30480839
Nat Mater. 2020 Jul;19(7):758-766
pubmed: 32341510
Nat Mater. 2020 Apr;19(4):428-435
pubmed: 31932670
ACS Comb Sci. 2011 Mar 14;13(2):126-34
pubmed: 21395341
Phys Chem Chem Phys. 2020 May 20;22(19):10764-10774
pubmed: 32159181
Nat Mater. 2011 Dec 15;11(1):19-29
pubmed: 22169914
Nature. 2015 Apr 16;520(7547):325-8
pubmed: 25849777
Small. 2021 Jun;17(25):e2007683
pubmed: 33893714