Ultra-narrow room-temperature emission from single CsPbBr


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
11 May 2022
Historique:
received: 18 08 2021
accepted: 25 03 2022
entrez: 13 5 2022
pubmed: 14 5 2022
medline: 14 5 2022
Statut: epublish

Résumé

Semiconductor quantum dots have long been considered artificial atoms, but despite the overarching analogies in the strong energy-level quantization and the single-photon emission capability, their emission spectrum is far broader than typical atomic emission lines. Here, by using ab-initio molecular dynamics for simulating exciton-surface-phonon interactions in structurally dynamic CsPbBr

Identifiants

pubmed: 35546149
doi: 10.1038/s41467-022-30016-0
pii: 10.1038/s41467-022-30016-0
pmc: PMC9095639
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

2587

Subventions

Organisme : Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung (Swiss National Science Foundation)
ID : Quantum Sciences and Technology NCCR.
Organisme : Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung (Swiss National Science Foundation)
ID : Quantum Sciences and Technology NCCR
Organisme : EC | Horizon 2020 Framework Programme (EU Framework Programme for Research and Innovation H2020)
ID : 819740

Informations de copyright

© 2022. The Author(s).

Références

J Am Chem Soc. 2017 Apr 19;139(15):5309-5312
pubmed: 28358191
ACS Nano. 2015 Sep 22;9(9):9106-16
pubmed: 26284384
J Am Chem Soc. 2018 Nov 21;140(46):15791-15803
pubmed: 30285448
Nano Lett. 2017 Nov 8;17(11):6838-6846
pubmed: 29039964
Nat Methods. 2012 Jun 28;9(7):676-82
pubmed: 22743772
ACS Nano. 2009 Sep 22;3(9):2487-94
pubmed: 19722505
Nature. 2018 Jan 10;553(7687):189-193
pubmed: 29323292
Science. 2019 Mar 8;363(6431):1068-1072
pubmed: 30792359
Nat Commun. 2015 Aug 20;6:8056
pubmed: 26290056
Nano Lett. 2018 Jun 13;18(6):3716-3722
pubmed: 29727576
ACS Energy Lett. 2019 Jan 11;4(1):63-74
pubmed: 30662955
Nano Lett. 2016 Jan 13;16(1):289-96
pubmed: 26636347
Nano Lett. 2021 Oct 27;21(20):8741-8748
pubmed: 34609148
Nano Lett. 2018 Jul 11;18(7):4061-4068
pubmed: 29927610
Nano Lett. 2015 Jun 10;15(6):3692-6
pubmed: 25633588
Science. 2000 Oct 13;290(5490):314-7
pubmed: 11030645
Nano Lett. 2015 Aug 12;15(8):5635-40
pubmed: 26207728
Nano Lett. 2019 Jun 12;19(6):3648-3653
pubmed: 31117751
Nanoscale. 2020 Jun 28;12(24):13113-13118
pubmed: 32584332
Nature. 2016 Mar 31;531(7596):618-22
pubmed: 26958836
Nature. 2018 Nov;563(7733):671-675
pubmed: 30405237
Chem Rev. 2019 Mar 13;119(5):3296-3348
pubmed: 30758194
Nature. 2014 May 1;509(7498):66-70
pubmed: 24784217
Nano Lett. 2018 Dec 12;18(12):7546-7551
pubmed: 30407011
J Phys Chem Lett. 2018 Apr 5;9(7):1561-1567
pubmed: 29518338
Science. 2019 Mar 15;363(6432):1199-1202
pubmed: 30872520
Nat Mater. 2018 May;17(5):394-405
pubmed: 29459748
Nature. 2017 Apr 6;544(7648):75-79
pubmed: 28321128
Science. 2016 Oct 7;354(6308):92-95
pubmed: 27846497
Chem Rev. 2010 Jan;110(1):389-458
pubmed: 19958036
Nat Mater. 2013 May;12(5):445-51
pubmed: 23377294
ACS Energy Lett. 2018 Mar 9;3(3):641-646
pubmed: 29552638
J Am Chem Soc. 2015 Aug 19;137(32):10276-81
pubmed: 26214734
Nano Lett. 2018 Apr 11;18(4):2233-2242
pubmed: 29498867
Nat Mater. 2019 Mar;18(3):249-255
pubmed: 30617342

Auteurs

Gabriele Rainò (G)

Department of Chemistry and Applied Biosciences, Institute of Inorganic Chemistry, ETH Zurich, 8093, Zurich, Switzerland. rainog@ethz.ch.
Laboratory for Thin Films and Photovoltaics, Empa-Swiss Federal Laboratories for Materials Science and Technology, CH-8600, Dübendorf, Switzerland. rainog@ethz.ch.

Nuri Yazdani (N)

Department of Information Technology and Electrical Engineering, ETH Zurich, Zurich, 8092, Switzerland.

Simon C Boehme (SC)

Department of Chemistry and Applied Biosciences, Institute of Inorganic Chemistry, ETH Zurich, 8093, Zurich, Switzerland.
Laboratory for Thin Films and Photovoltaics, Empa-Swiss Federal Laboratories for Materials Science and Technology, CH-8600, Dübendorf, Switzerland.
Department of Theoretical Chemistry, Faculty of Science, Vrije Universiteit Amsterdam, 1081 HV, Amsterdam, The Netherlands.

Manuel Kober-Czerny (M)

Department of Chemistry and Applied Biosciences, Institute of Inorganic Chemistry, ETH Zurich, 8093, Zurich, Switzerland.
Laboratory for Thin Films and Photovoltaics, Empa-Swiss Federal Laboratories for Materials Science and Technology, CH-8600, Dübendorf, Switzerland.

Chenglian Zhu (C)

Department of Chemistry and Applied Biosciences, Institute of Inorganic Chemistry, ETH Zurich, 8093, Zurich, Switzerland.
Laboratory for Thin Films and Photovoltaics, Empa-Swiss Federal Laboratories for Materials Science and Technology, CH-8600, Dübendorf, Switzerland.

Franziska Krieg (F)

Department of Chemistry and Applied Biosciences, Institute of Inorganic Chemistry, ETH Zurich, 8093, Zurich, Switzerland.
Laboratory for Thin Films and Photovoltaics, Empa-Swiss Federal Laboratories for Materials Science and Technology, CH-8600, Dübendorf, Switzerland.

Marta D Rossell (MD)

Electron Microscopy Center, Empa-Swiss Federal Laboratories for Materials Science and Technology, CH-8600, Dübendorf, Switzerland.

Rolf Erni (R)

Electron Microscopy Center, Empa-Swiss Federal Laboratories for Materials Science and Technology, CH-8600, Dübendorf, Switzerland.

Vanessa Wood (V)

Department of Information Technology and Electrical Engineering, ETH Zurich, Zurich, 8092, Switzerland.

Ivan Infante (I)

Department of Theoretical Chemistry, Faculty of Science, Vrije Universiteit Amsterdam, 1081 HV, Amsterdam, The Netherlands.
Department of Nanochemistry, Istituto Italiano di Tecnologia, Via Morego 30, 16163, Genova, Italy.

Maksym V Kovalenko (MV)

Department of Chemistry and Applied Biosciences, Institute of Inorganic Chemistry, ETH Zurich, 8093, Zurich, Switzerland. mvkovalenko@ethz.ch.
Laboratory for Thin Films and Photovoltaics, Empa-Swiss Federal Laboratories for Materials Science and Technology, CH-8600, Dübendorf, Switzerland. mvkovalenko@ethz.ch.

Classifications MeSH