New Mechanism for Long Photo-Induced Enhanced Raman Spectroscopy in Au Nanoparticles Embedded in TiO

TiO 2 cathodoluminescence nanoparticles photo-induced charge separation photo-induced enhanced Raman spectroscopy surface enhanced Raman spectroscopy

Journal

Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338

Informations de publication

Date de publication:
Jun 2022
Historique:
revised: 27 04 2022
received: 18 02 2022
pubmed: 27 5 2022
medline: 27 5 2022
entrez: 26 5 2022
Statut: ppublish

Résumé

The photo-induced enhanced Raman spectroscopy (PIERS) effect is a phenomenon taking place when plasmonic nanoparticles deposited on a semiconductor are illuminated by UV light prior to Raman measurement. Results from the literature show that the PIERS effect lasts for about an hour. The proposed mechanism for this effect is the creation of oxygen vacancies in the semiconductor that would create a path for charge transfer between the analyte and the nanoparticles. However, this hypothesis has never been confirmed experimentally. Furthermore, the tested structure of the PIERS substrate has always been composed of plasmonic nanoparticles deposited on top of the semiconductor. Here, gold nanoparticles co-deposited with porous TiO

Identifiants

pubmed: 35616163
doi: 10.1002/smll.202201088
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2201088

Informations de copyright

© 2022 Wiley-VCH GmbH.

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Auteurs

Andrea Brognara (A)

Dipartimento di Energia, Micro and Nanostructured Materials Laboratory, Politecnico di Milano, via Ponzio 34/3, Milano, I-20133, Italy.
Department of Structure and Nano/-Micromechanics of Materials, Max-Planck-Institut für Eisenforschung GmbH, Max-Planck-Straße 1, 40237, Düsseldorf, Germany.

Beatrice R Bricchi (BR)

Dipartimento di Energia, Micro and Nanostructured Materials Laboratory, Politecnico di Milano, via Ponzio 34/3, Milano, I-20133, Italy.

Ludovic William (L)

Laboratoire des Sciences des Procédés et des Matériaux (LSPM), CNRS, Université Sorbonne Paris Nord, Villetaneuse, 93430, France.

Ovidiu Brinza (O)

Laboratoire des Sciences des Procédés et des Matériaux (LSPM), CNRS, Université Sorbonne Paris Nord, Villetaneuse, 93430, France.

Maria Konstantakopoulou (M)

Laboratoire des Sciences des Procédés et des Matériaux (LSPM), CNRS, Université Sorbonne Paris Nord, Villetaneuse, 93430, France.

Andrea Li Bassi (AL)

Dipartimento di Energia, Micro and Nanostructured Materials Laboratory, Politecnico di Milano, via Ponzio 34/3, Milano, I-20133, Italy.

Matteo Ghidelli (M)

Dipartimento di Energia, Micro and Nanostructured Materials Laboratory, Politecnico di Milano, via Ponzio 34/3, Milano, I-20133, Italy.
Department of Structure and Nano/-Micromechanics of Materials, Max-Planck-Institut für Eisenforschung GmbH, Max-Planck-Straße 1, 40237, Düsseldorf, Germany.
Laboratoire des Sciences des Procédés et des Matériaux (LSPM), CNRS, Université Sorbonne Paris Nord, Villetaneuse, 93430, France.

Nathalie Lidgi-Guigui (N)

Laboratoire des Sciences des Procédés et des Matériaux (LSPM), CNRS, Université Sorbonne Paris Nord, Villetaneuse, 93430, France.

Classifications MeSH