Oxocarbenium ion cyclizations for the synthesis of disaccharide mimetics of 2-amino-2-deoxy-pyranosides: Application to the carbasugar of β-galactosamine-(1,4)-3-O-methyl-D-chiro-inositol.

4-C-Lyxose Carbadisaccharide Galactosamine Glycomimetic Inositol Insulin

Journal

Carbohydrate research
ISSN: 1873-426X
Titre abrégé: Carbohydr Res
Pays: Netherlands
ID NLM: 0043535

Informations de publication

Date de publication:
Aug 2022
Historique:
received: 18 03 2022
revised: 14 05 2022
accepted: 16 05 2022
pubmed: 2 6 2022
medline: 22 6 2022
entrez: 1 6 2022
Statut: ppublish

Résumé

The synthesis of the carbasugar of β-galactosamine-(1,4)-3-O-methyl-D-chiro-inositol (INS-2), a potential tool for studying glucose metabolism, is described. The synthetic strategy, entails an oxocarbenium ion cyclization on a chiro-inositol derived, thioacetal-enol ether to give a carbocyclic enol ether, which is elaborated to the 2-amino-2-deoxy carbasugar framework via a 2-oximo derivative.

Identifiants

pubmed: 35643049
pii: S0008-6215(22)00096-9
doi: 10.1016/j.carres.2022.108595
pii:
doi:

Substances chimiques

Carbasugars 0
Disaccharides 0
Ethers 0
Inositol 4L6452S749
Galactosamine 7535-00-4

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

108595

Informations de copyright

Copyright © 2022 Elsevier Ltd. All rights reserved.

Auteurs

Sunej K Hans (SK)

Department of Chemistry, Hunter College and The Graduate Center of the City University of New York, New York, NY, 10016, USA.

Steven Truong (S)

Department of Chemistry, Hunter College and The Graduate Center of the City University of New York, New York, NY, 10016, USA.

David R Mootoo (DR)

Department of Chemistry, Hunter College and The Graduate Center of the City University of New York, New York, NY, 10016, USA. Electronic address: dmootoo@hunter.cuny.edu.

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Classifications MeSH