The Potential of Sewage Sludge to Predict and Evaluate the Human Chemical Exposome.


Journal

Environmental science & technology letters
ISSN: 2328-8930
Titre abrégé: Environ Sci Technol Lett
Pays: United States
ID NLM: 101628367

Informations de publication

Date de publication:
14 Dec 2021
Historique:
received: 19 10 2021
revised: 05 11 2021
accepted: 08 11 2021
entrez: 1 6 2022
pubmed: 2 6 2022
medline: 2 6 2022
Statut: ppublish

Résumé

Chemicals are part of our daily lives, and we are exposed to numerous chemicals through multiple pathways. Relevant scientific evidence contributing to the regulation of hazardous chemicals require a holistic approach to assess simultaneous exposure to multiple compounds. Biomonitoring provides an accurate estimation of exposure to chemicals through very complex and costly sampling campaigns. Finding efficient proxies to predict the risk of chemical exposure in humans is an urgent need to cover large areas and populations at a reasonable cost. We conducted an exploratory study to characterize the human chemical exposome in maternal blood and placenta samples of a population-based birth cohort in Barcelona (2018-2021). Ultimate HRMS-based approaches were applied including wide-scope target, suspect, and nontarget screening. Forty-two chemicals were identified including pesticides, personal care products, or industrial compounds, among others, in the range of ng/mL and ng/g. In parallel, sewage sludge from the wastewater treatment plants serving the residence areas of the studied population were also screened, showing correlations with the type and concentrations of chemicals found in humans. Our findings were suggestive for the potential use of sewage sludge as a proxy of the human exposure and its application in early warning systems to prevent bioaccumulation of hazardous chemicals.

Identifiants

pubmed: 35647215
doi: 10.1021/acs.estlett.1c00848
pmc: PMC9132361
doi:

Types de publication

Journal Article

Langues

eng

Pagination

1077-1084

Informations de copyright

© 2021 American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

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Auteurs

Ruben Gil-Solsona (R)

Department of Environmental Chemistry, Institute of Environmental Assessment and Water Research - Severo Ochoa Excellence Center (IDAEA), Spanish Council of Scientific Research (CSIC), Jordi Girona 18-26, Barcelona 08034, Spain.

Maria-Christina Nika (MC)

Laboratory of Analytical Chemistry, Department of Chemistry, National and Kapodistrian University of Athens, Panepistimiopolis Zografou, Athens 15771, Greece.

Mariona Bustamante (M)

ISGlobal, Barcelona 08003, Spain.
Universitat Pompeu Fabra (UPF), Barcelona 08003, Spain.
CIBER Epidemiología y Salud Pública (CIBERESP), Madrid 28029, Spain.

Cristina M Villanueva (CM)

ISGlobal, Barcelona 08003, Spain.
Universitat Pompeu Fabra (UPF), Barcelona 08003, Spain.
CIBER Epidemiología y Salud Pública (CIBERESP), Madrid 28029, Spain.
IMIM (Hospital del Mar Medical Research Institute), Doctor Aiguader 88, Barcelona 08003, Spain.

Maria Foraster (M)

ISGlobal, Barcelona 08003, Spain.
Universitat Pompeu Fabra (UPF), Barcelona 08003, Spain.
CIBER Epidemiología y Salud Pública (CIBERESP), Madrid 28029, Spain.
PHAGEX Research Group, Blanquerna School of Health Science, Universitat Ramon Llull (URL), Carrer de Padilla, 326, Barcelona 08025, Spain.

Marta Cosin-Tomás (M)

Department of Human Genetics, Research Institute of the McGill University Health Center, McGill University, 845 Sherbrooke St W, Montreal, Quebec H3A 0G4, Canada.

Nikiforos Alygizakis (N)

Laboratory of Analytical Chemistry, Department of Chemistry, National and Kapodistrian University of Athens, Panepistimiopolis Zografou, Athens 15771, Greece.

Maria Dolores Gómez-Roig (MD)

BCNatal - Barcelona Center for Maternal Fetal and Neonatal Medicine (Hospital Sant Joan de Déu and Hospital Clínic), University of Barcelona, Esplugues de Llobregat, Passeig de Sant Joan de Déu, 2, Barcelona 08950, Spain.

Elisa Llurba-Olive (E)

Maternal and Fetal Medicine Unit, Obstetrics and Gynecology Department, Sant Pau University Hospital, C. de Villarroel, 170, Barcelona 08036, Spain.
Development Network (SAMID), RD16/0022/0015, Instituto de Salud Carlos III, Av. de Monforte de Lemos, 5, Madrid 28029, Spain.

Jordi Sunyer (J)

ISGlobal, Barcelona 08003, Spain.
Universitat Pompeu Fabra (UPF), Barcelona 08003, Spain.
CIBER Epidemiología y Salud Pública (CIBERESP), Madrid 28029, Spain.

Nikolaos S Thomaidis (NS)

Laboratory of Analytical Chemistry, Department of Chemistry, National and Kapodistrian University of Athens, Panepistimiopolis Zografou, Athens 15771, Greece.

Payam Dadvand (P)

ISGlobal, Barcelona 08003, Spain.
Universitat Pompeu Fabra (UPF), Barcelona 08003, Spain.
CIBER Epidemiología y Salud Pública (CIBERESP), Madrid 28029, Spain.

Pablo Gago-Ferrero (P)

Department of Environmental Chemistry, Institute of Environmental Assessment and Water Research - Severo Ochoa Excellence Center (IDAEA), Spanish Council of Scientific Research (CSIC), Jordi Girona 18-26, Barcelona 08034, Spain.

Classifications MeSH