Comparative Evaluation of Light-Driven Catalysis: A Framework for Standardized Reporting of Data.
Comparability
Heterogeneous
Homogeneous
Light-Driven Catalysis
Photocatalysis
Journal
Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543
Informations de publication
Date de publication:
11 Jul 2022
11 Jul 2022
Historique:
received:
18
10
2021
pubmed:
14
6
2022
medline:
14
6
2022
entrez:
13
6
2022
Statut:
ppublish
Résumé
Light-driven homogeneous and heterogeneous catalysis require a complex interplay between light absorption, charge separation, charge transfer, and catalytic turnover. Optical and irradiation parameters as well as reaction engineering aspects play major roles in controlling catalytic performance. This multitude of factors makes it difficult to objectively compare light-driven catalysts and provide an unbiased performance assessment. This Scientific Perspective highlights the importance of collecting and reporting experimental data in homogeneous and heterogeneous light-driven catalysis. A critical analysis of the benefits and limitations of the commonly used experimental indicators is provided. Data collection and reporting according to FAIR principles is discussed in the context of future automated data analysis. The authors propose a minimum dataset as a basis for unified collecting and reporting of experimental data in homogeneous and heterogeneous light-driven catalysis. The community is encouraged to support the future development of this parameter list through an open online repository.
Identifiants
pubmed: 35698245
doi: 10.1002/anie.202114106
pmc: PMC9401044
doi:
Types de publication
Journal Article
Review
Langues
eng
Sous-ensembles de citation
IM
Pagination
e202114106Subventions
Organisme : Deutsche Forschungsgemeinschaft
ID : 364549901; 359737763; 404382951; 404530119
Organisme : Vector Stiftung
ID : P2019-0110
Informations de copyright
© 2022 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH.
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