Transcriptional Perturbations of 2,6-Diaminopurine and 2-Aminopurine.


Journal

ACS chemical biology
ISSN: 1554-8937
Titre abrégé: ACS Chem Biol
Pays: United States
ID NLM: 101282906

Informations de publication

Date de publication:
15 07 2022
Historique:
pubmed: 15 6 2022
medline: 19 7 2022
entrez: 14 6 2022
Statut: ppublish

Résumé

2,6-Diaminopurine (Z) is a naturally occurring adenine (A) analog that bacteriophages employ in place of A in their genetic alphabet. Recent discoveries of biogenesis pathways of Z in bacteriophages have stimulated substantial research interest in this DNA modification. Here, we systematically examined the effects of Z on the efficiency and fidelity of DNA transcription. Our results showed that Z exhibited no mutagenic yet substantial inhibitory effects on transcription mediated by purified T7 RNA polymerase and by human RNA polymerase II in HeLa nuclear extracts and in human cells. A structurally related adenine analog, 2-aminopurine (2AP), strongly blocked T7 RNA polymerase but did not impede human RNA polymerase II

Identifiants

pubmed: 35700389
doi: 10.1021/acschembio.2c00369
pmc: PMC9354233
mid: NIHMS1827269
doi:

Substances chimiques

2-Aminopurine 452-06-2
2,6-diaminopurine 49P95BAU4Z
DNA 9007-49-2
RNA Polymerase II EC 2.7.7.-

Types de publication

Journal Article Research Support, Non-U.S. Gov't Research Support, N.I.H., Extramural

Langues

eng

Sous-ensembles de citation

IM

Pagination

1672-1676

Subventions

Organisme : NCI NIH HHS
ID : P01 CA092584
Pays : United States
Organisme : NIEHS NIH HHS
ID : R35 ES031707
Pays : United States

Références

Nat Rev Mol Cell Biol. 2014 Jul;15(7):465-81
pubmed: 24954209
Mutagenesis. 1997 Jul;12(4):277-83
pubmed: 9237774
Trends Biochem Sci. 2006 Feb;31(2):89-97
pubmed: 16403636
Mol Cell Biol. 2010 Jul;30(13):3206-15
pubmed: 20421413
Nature. 1977 Nov 24;270(5635):369-70
pubmed: 413053
FEBS Lett. 1987 Sep 28;222(1):89-94
pubmed: 2820801
J Biol Chem. 2002 Oct 25;277(43):40640-9
pubmed: 12189135
Nat Rev Cancer. 2011 Mar;11(3):218-27
pubmed: 21346784
Nucleic Acids Res. 2014 Dec 16;42(22):13706-13
pubmed: 25404131
Science. 2021 Apr 30;372(6541):516-520
pubmed: 33926955
Chem Rev. 2006 Feb;106(2):474-88
pubmed: 16464015
Science. 2021 Apr 30;372(6541):512-516
pubmed: 33926954
Science. 2021 Apr 30;372(6541):520-524
pubmed: 33926956
Nature. 1990 Jan 4;343(6253):33-7
pubmed: 1688644
Biochemistry. 2011 Nov 22;50(46):10136-49
pubmed: 22023103
Proc Natl Acad Sci U S A. 1986 Aug;83(15):5434-8
pubmed: 3461441
Nat Protoc. 2015 Sep;10(9):1389-406
pubmed: 26292071
Proc Natl Acad Sci U S A. 2008 Dec 2;105(48):18877-82
pubmed: 19020090
Nat Commun. 2021 Dec 1;12(1):7001
pubmed: 34853308
Nucleic Acids Res. 2019 Sep 19;47(16):8537-8547
pubmed: 31226203
Bioessays. 1999 May;21(5):402-11
pubmed: 10376011
Nat Chem Biol. 2012 Oct;8(10):817-22
pubmed: 22902614
Angew Chem Int Ed Engl. 2021 May 3;60(19):10775-10783
pubmed: 33325148
Sci Transl Med. 2013 Aug 7;5(197):197ra102
pubmed: 23926200
Nat Commun. 2021 Aug 5;12(1):4710
pubmed: 34354070
J Am Chem Soc. 2021 Oct 6;143(39):16197-16205
pubmed: 34555898
Nat Commun. 2021 May 21;12(1):3018
pubmed: 34021158
Proc Natl Acad Sci U S A. 2020 Apr 28;117(17):9338-9348
pubmed: 32284409
J Cell Physiol. 2013 Dec;228(12):2257-61
pubmed: 23696333
Nature. 2021 Oct;598(7880):368-372
pubmed: 34526721
Nat Rev Mol Cell Biol. 2008 Dec;9(12):958-70
pubmed: 19023283
Proc Natl Acad Sci U S A. 2011 Aug 23;108(34):13995-8
pubmed: 21836052
Nucleic Acids Res. 2012 Mar;40(6):2494-505
pubmed: 22121226
Chembiochem. 2015 May 26;16(8):1212-8
pubmed: 25881991
Helv Chim Acta. 1999 Nov;82(11):1799-805
pubmed: 11543571
Nat Commun. 2021 Apr 23;12(1):2420
pubmed: 33893297

Auteurs

Jiyeong Park (J)

Center for Genomic Integrity, Institute for Basic Science, Ulsan 44919, Republic of Korea.

Hyun Suk Kim (HS)

Center for Genomic Integrity, Institute for Basic Science, Ulsan 44919, Republic of Korea.

Orlando D Schärer (OD)

Center for Genomic Integrity, Institute for Basic Science, Ulsan 44919, Republic of Korea.
Department of Biological Sciences, Ulsan National Institute of Science and Technology (UNIST), Ulsan, 44919, Republic of Korea.

Articles similaires

[Redispensing of expensive oral anticancer medicines: a practical application].

Lisanne N van Merendonk, Kübra Akgöl, Bastiaan Nuijen
1.00
Humans Antineoplastic Agents Administration, Oral Drug Costs Counterfeit Drugs

Smoking Cessation and Incident Cardiovascular Disease.

Jun Hwan Cho, Seung Yong Shin, Hoseob Kim et al.
1.00
Humans Male Smoking Cessation Cardiovascular Diseases Female
Humans United States Aged Cross-Sectional Studies Medicare Part C
1.00
Humans Yoga Low Back Pain Female Male

Classifications MeSH