Electronic Modulation of Ru Nanosheet by d-d Orbital Coupling for Enhanced Hydrogen Oxidation Reaction in Alkaline Electrolytes.
Ru
alkaline polymer electrolyte fuel cells
conduction band minimum
d-d orbital coupling
hydrogen oxidation reaction
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
Jul 2022
Jul 2022
Historique:
revised:
02
06
2022
received:
18
04
2022
pubmed:
28
6
2022
medline:
28
6
2022
entrez:
27
6
2022
Statut:
ppublish
Résumé
The alkaline polymer electrolyte fuel cells (APEFCs) hold great promise for using nonnoble metal-based electrocatalysts toward the cathodic oxygen reduction reaction (ORR), but are hindered by the sluggish anodic hydrogen oxidation reaction (HOR) in alkaline electrolytes. Here, a strategy is reported to promote the alkaline HOR performance of Ru by incorporating 3d-transition metals (V, Fe, Co, and Ni), where the conduction band minimum (CBM) level of Ru can be rationally tailored through strong d-d orbital coupling. As expected, the obtained RuFe nanosheet exhibits outstanding HOR performance with the mass activity of 233.46 A g
Identifiants
pubmed: 35754182
doi: 10.1002/smll.202202404
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2202404Subventions
Organisme : National Key Research and Development program of China
ID : 2018YFB1502302
Organisme : National Key Research and Development program of China
ID : 2021YFB4001200
Organisme : National Natural Science Foundation of China
ID : 21972107
Organisme : Fundamental Research Funds for the Central Universities
ID : 2042022kf1179
Organisme : Natural Science Foundation of Jiangsu Province
ID : BK20191186
Organisme : Natural Science Foundation of Hubei Province
ID : 2020CFA095
Informations de copyright
© 2022 Wiley-VCH GmbH.
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