Zn(ii)-Coordination-driven self-assembled nanoagents for multimodal imaging-guided photothermal/gene synergistic therapy.


Journal

Chemical science
ISSN: 2041-6520
Titre abrégé: Chem Sci
Pays: England
ID NLM: 101545951

Informations de publication

Date de publication:
22 Jun 2022
Historique:
received: 28 03 2022
accepted: 01 06 2022
entrez: 8 7 2022
pubmed: 9 7 2022
medline: 9 7 2022
Statut: epublish

Résumé

Synergistic photothermal therapy (PTT) with gene therapy (GT) has drawn emerging interest in the improvement of cancer therapeutic efficiency, while the co-delivery of photothermal agents (PTAs) and therapeutic genes by an integrated nanoplatform, with controllability and biodegradability, is still challenging and urgently desired. Herein, a multi-functional metal-organic framework (MOF) based PTT-GT platform (siRNA@PT-ZIF-8) was developed, which was constructed with siRNA, a near-infrared (NIR) responsive organic dye IR780 derivative (IR780-1), and 2-methylimidazole (2-MIM) by a facile one-pot self-assembly method. This "all-in-one" system of siRNA@PT-ZIF-8 enabled not only photothermal/photoacoustic/fluorescence multimodal imaging but also tumor microenvironment responsiveness for specific and on-demand release of therapeutic cargos, overcoming the inherent limitations of free gene or organic PTA molecules (

Identifiants

pubmed: 35799809
doi: 10.1039/d2sc01769e
pii: d2sc01769e
pmc: PMC9214881
doi:

Types de publication

Journal Article

Langues

eng

Pagination

7355-7364

Informations de copyright

This journal is © The Royal Society of Chemistry.

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

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Auteurs

Hui Hu (H)

Key Laboratory of Chem-Biosensing of Anhui Province, Key Laboratory of Functional Molecular Solids, College of Chemistry and Materials Science, Anhui Normal University Wuhu 241000 Anhui Province China wangyuz@mail.ahnu.edu.cn.

Nan Yang (N)

Key Laboratory of Flexible Electronics (KLOFE), Institute of Advanced Materials (IAM), Nanjing Tech University (NanjingTech) Nanjing 211816 China iamxcdong@njtech.edu.cn.

Jiahui Sun (J)

Key Laboratory of Chem-Biosensing of Anhui Province, Key Laboratory of Functional Molecular Solids, College of Chemistry and Materials Science, Anhui Normal University Wuhu 241000 Anhui Province China wangyuz@mail.ahnu.edu.cn.

Fu Zhou (F)

Key Laboratory of Chem-Biosensing of Anhui Province, Key Laboratory of Functional Molecular Solids, College of Chemistry and Materials Science, Anhui Normal University Wuhu 241000 Anhui Province China wangyuz@mail.ahnu.edu.cn.

Rui Gu (R)

Key Laboratory of Flexible Electronics (KLOFE), Institute of Advanced Materials (IAM), Nanjing Tech University (NanjingTech) Nanjing 211816 China iamxcdong@njtech.edu.cn.

Yuan Liu (Y)

Key Laboratory of Chem-Biosensing of Anhui Province, Key Laboratory of Functional Molecular Solids, College of Chemistry and Materials Science, Anhui Normal University Wuhu 241000 Anhui Province China wangyuz@mail.ahnu.edu.cn.

Li Wang (L)

Key Laboratory of Chem-Biosensing of Anhui Province, Key Laboratory of Functional Molecular Solids, College of Chemistry and Materials Science, Anhui Normal University Wuhu 241000 Anhui Province China wangyuz@mail.ahnu.edu.cn.

Xuejiao Song (X)

Key Laboratory of Flexible Electronics (KLOFE), Institute of Advanced Materials (IAM), Nanjing Tech University (NanjingTech) Nanjing 211816 China iamxcdong@njtech.edu.cn.

Ruirui Yun (R)

Key Laboratory of Chem-Biosensing of Anhui Province, Key Laboratory of Functional Molecular Solids, College of Chemistry and Materials Science, Anhui Normal University Wuhu 241000 Anhui Province China wangyuz@mail.ahnu.edu.cn.

Xiaochen Dong (X)

Key Laboratory of Flexible Electronics (KLOFE), Institute of Advanced Materials (IAM), Nanjing Tech University (NanjingTech) Nanjing 211816 China iamxcdong@njtech.edu.cn.

Guangfeng Wang (G)

Key Laboratory of Chem-Biosensing of Anhui Province, Key Laboratory of Functional Molecular Solids, College of Chemistry and Materials Science, Anhui Normal University Wuhu 241000 Anhui Province China wangyuz@mail.ahnu.edu.cn.

Classifications MeSH