Multicomponent, Functionalized HKUST-1 Analogues Assembled via Reticulation of Prefabricated Metal-Organic Polyhedral Cavities.


Journal

Journal of the American Chemical Society
ISSN: 1520-5126
Titre abrégé: J Am Chem Soc
Pays: United States
ID NLM: 7503056

Informations de publication

Date de publication:
31 Aug 2022
Historique:
pubmed: 17 8 2022
medline: 17 8 2022
entrez: 16 8 2022
Statut: ppublish

Résumé

Metal-organic frameworks (MOFs) assembled from multiple building blocks exhibit greater chemical complexity and superior functionality in practical applications. Herein, we report a new approach based on using prefabricated cavities to design isoreticular multicomponent MOFs from a known parent MOF. We demonstrate this concept with the formation of multicomponent HKUST-1 analogues, using a prefabricated cavity that comprises a cuboctahedral Rh(II) metal-organic polyhedron functionalized with 24 carboxylic acid groups. The cavities are reticulated in three dimensions via Cu(II)-paddlewheel clusters and (functionalized) 1,3,5-benzenetricarboxylate linkers to form three- and four-component HKUST-1 analogues.

Identifiants

pubmed: 35973046
doi: 10.1021/jacs.2c06131
pmc: PMC9437915
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

15745-15753

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Auteurs

Akim Khobotov-Bakishev (A)

Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain.
Departament de Química, Facultat de Ciències, Universitat Autònoma de Barcelona, 08193 Bellaterra, Spain.

Cornelia von Baeckmann (C)

Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain.
Departament de Química, Facultat de Ciències, Universitat Autònoma de Barcelona, 08193 Bellaterra, Spain.

Borja Ortín-Rubio (B)

Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain.
Departament de Química, Facultat de Ciències, Universitat Autònoma de Barcelona, 08193 Bellaterra, Spain.

Laura Hernández-López (L)

Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain.
Departament de Química, Facultat de Ciències, Universitat Autònoma de Barcelona, 08193 Bellaterra, Spain.

Alba Cortés-Martínez (A)

Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain.
Departament de Química, Facultat de Ciències, Universitat Autònoma de Barcelona, 08193 Bellaterra, Spain.

Jordi Martínez-Esaín (J)

Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain.

Felipe Gándara (F)

Consejo Superior de Investigaciones Científicas (CSIC), Materials Science Institute of Madrid (ICMM), Calle Sor Juana Inés de la Cruz, 3, 28049 Madrid, Spain.

Judith Juanhuix (J)

ALBA Synchrotron, Carrer de la Llum, 2, 26, 08290 Cerdanyola del Vallès, Barcelona, Spain.

Ana E Platero-Prats (AE)

Departamento de Química Inorgánica, Facultad de Ciencias, Universidad Autónoma de Madrid, 28049 Madrid, Spain.
Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, 28049 Madrid, Spain.

Jordi Faraudo (J)

Institut de Ciència de Materials de Barcelona (ICMAB-CSIC), 08193 Bellaterra, Spain.

Arnau Carné-Sánchez (A)

Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain.
Departament de Química, Facultat de Ciències, Universitat Autònoma de Barcelona, 08193 Bellaterra, Spain.

Daniel Maspoch (D)

Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain.
Departament de Química, Facultat de Ciències, Universitat Autònoma de Barcelona, 08193 Bellaterra, Spain.
ICREA, Pg. Lluís Companys 23, 08010 Barcelona, Spain.

Classifications MeSH